Tracer tests - possibilities and limitations. Experience from SKB fieldwork: 1977-2007

Tracer tests have played, and still play, a central role in investigations relating to the understanding of radionuclide retention processes in the field. At present there is a debate within the scientific community concerning how, and to what extent, tracer tests can be used to evaluate large-scale and long-term transport and retardation of radionuclides and other solutes of interest for Safety Assessment of repositories for spent nuclear fuel. In this report the SKB fieldwork on tracer tests performed at Swedish sites from 1977 to 2007 is described and discussed. Furthermore, the knowledge and process understanding evolved during the decades of radionuclide transport experiments and modelling within the SKB programme is summarised. One of the main objectives of this report is to discuss what data and knowledge can be extracted from different in situ tests in a robust fashion. Given the level of complexity associated with transport processes that may occur over the timescale of a tracer test, the utility of tracer tests is considered in the context of evidence-based interpretations of data which we characterise in the form of a sequence of questions of increasing complexity. The complexity of this sequence ranges from whether connection can be confirmed between injection and withdrawal points to whether quantitative data can be extrapolated from a tracer test to be subsequently used in Safety Assessment. The main findings of this report are that: Field scale tracer tests can confirm flow connectivity. Field scale tracer tests confirm the existence of retention. Field scale tracer tests alone can only broadly substantiate our process understanding. However, if performing extensive Site Characterisation and integrating the tracer test results with the full range of geoscientific information available, much support can be given to our process understanding. Field scale tracer tests can deliver the product of the material property group MPG and the F-factor, valid only for the tracer test configuration, but not separate them without introducing additional assumptions. Field scale tracer tests (in flowing fractures) alone cannot deliver individual transport parameters, such as effective diffusivity, flow-wetted surface, etc in the absence of additional supporting information. Lumped or individual transport parameters obtained from inverse modelling of tracer test data are not directly transferable to Safety Assessment flow conditions or timescales. In addition to the above findings, another objective of this report has been to describe and highlight a number of elaborate in situ tracer tests that SKB has performed and reported. Many of these experiments have contributed immeasurably to current process understanding although may not be widely known to the general reader