A segmented cell approach for studying the effects of serpentine flow field parameters on PEMFC current distribution
- 1. Hawaii Natural Energy Institute, University of Hawaii, 1680 East-West Road, POST 109, Honolulu, HI 96822 (United States)
- 2. National Renewable Energy Laboratory, 1617 Cole Blvd., Golden, CO 80401-3305 (United States)
Description
Highlights: ► Effects of a flow field design on PEMFC were investigated. ► A segmented cell was used to study 6- and 10-channel serpentine flow fields. ► 10-Channel flow field improved a fuel cell's performance at high current. ► Performance distribution was more uniform for 10-channel than for 6-channel flow field. ► The performance improvement was due to an increased pressure drop. -- Abstract: A serpentine flow field is a commonly used design in proton exchange membrane fuel cells (PEMFCs). Consequently, optimization of the flow field parameters is critically needed. A segmented cell system was used to study the impact of the flow field's parameters on the current distribution in a PEMFC, and the data obtained were analyzed in terms of voltage overpotentials. 6-Channel and 10-channel serpentine flow field designs were investigated. At low current the segments performance was found to slightly decrease for a 10-channel serpentine flow field. However, increasing the number of channels increased the fuel cell performance when operating at high current and the cell performance became more uniform downstream. The observed improvement in fuel cell performance was attributed to a decrease in mass transfer voltage losses (permeability and diffusion), due to an increased pressure drop. Spatially distributed electrochemical impedance spectroscopy (EIS) data showed differences in the local segment impedance response and confirmed the performance distribution and the impact of the flow field design
Availability note (English)
Available from http://dx.doi.org/10.1016/j.electacta.2012.10.103Additional details
Identifiers
- DOI
- 10.1016/j.electacta.2012.10.103;
- PII
- S0013-4686(12)01717-3;
Publishing Information
- Journal Title
- Electrochimica Acta
- Journal Volume
- 88
- Journal Page Range
- p. 571-579
- ISSN
- 0013-4686
- CODEN
- ELCAAV
INIS
- Country of Publication
- United Kingdom
- Country of Input or Organization
- International Atomic Energy Agency (IAEA)
- INIS RN
- 45059603
- Subject category
- S37: INORGANIC, ORGANIC, PHYSICAL AND ANALYTICAL CHEMISTRY;
- Descriptors DEI
- DISTRIBUTION; ELECTRIC POTENTIAL; MASS TRANSFER; OPTIMIZATION; PERMEABILITY; PRESSURE DROP; PROTON EXCHANGE MEMBRANE FUEL CELLS; SERPENTINE; SPECTROSCOPY
- Descriptors DEC
- DIRECT ENERGY CONVERTERS; ELECTROCHEMICAL CELLS; FUEL CELLS; MINERALS; PHYSICAL PROPERTIES; SILICATE MINERALS; SOLID ELECTROLYTE FUEL CELLS
Optional Information
- Copyright
- Copyright (c) 2012 Elsevier Science B.V., Amsterdam, The Netherlands, All rights reserved.