Published October 14, 2012
| Version v1
Journal article
Molecular-frame photoelectron angular distribution imaging studies of OCS S1s photoionization
Creators
- 1. UPMC, Université Paris 06, LCPMR, 11 rue Pierre et Marie Curie, 75231 Paris Cedex 05 (France)
- 2. Synchrotron SOLEIL, l'Orme des Merisiers, Saint-Aubin, BP 48, 91192 Gif-sur-Yvette Cedex (France)
- 3. Dipartimento di Scienze Chimiche, Università di Trieste, Via L Giorgieri 1, I-34127 Trieste (Italy)
Description
Molecular-frame photoelectron angular distributions (MFPADs) in carbonyl sulfide at selected photon energies above the sulfur 1s ionization threshold have been measured using a recently developed vector-correlation experimental setup and theoretically calculated using the time-dependent DFT method. For this linear molecule, the selection of the fragmentation channel CO+ + S+ is an effective method to fix the molecular frame. The experimental results are found in good agreement with the calculated MFPADs.
Availability note (English)
Available from http://dx.doi.org/10.1088/0953-4075/45/19/194005Additional details
Identifiers
Publishing Information
- Journal Title
- Journal of Physics. B, Atomic, Molecular and Optical Physics
- Journal Volume
- 45
- Journal Issue
- 19
- Journal Page Range
- [12 p.]
- ISSN
- 0953-4075
- CODEN
- JPAPEH
INIS
- Country of Publication
- United Kingdom
- Country of Input or Organization
- International Atomic Energy Agency (IAEA)
- INIS RN
- 44038356
- Subject category
- S74: ATOMIC AND MOLECULAR PHYSICS;
- Descriptors DEI
- ANGULAR DISTRIBUTION; CARBON OXIDES; CARBON OXYSULFIDE; COMPUTERIZED SIMULATION; CORRELATIONS; DENSITY FUNCTIONAL METHOD; FRAGMENTATION; MOLECULAR IONS; MOLECULES; PHOTOIONIZATION; PHOTONS; S STATES; SULFUR IONS; TIME DEPENDENCE
- Descriptors DEC
- BOSONS; CALCULATION METHODS; CARBON COMPOUNDS; CHALCOGENIDES; CHARGED PARTICLES; DISTRIBUTION; ELEMENTARY PARTICLES; ENERGY LEVELS; IONIZATION; IONS; MASSLESS PARTICLES; OXIDES; OXYGEN COMPOUNDS; SIMULATION; SULFUR COMPOUNDS; VARIATIONAL METHODS