Published April 19, 2024 | Version v1
Journal article

Non-Fermi liquid and Hund correlation in La4Ni3O10 under high pressure

  • 1. Department of Physics and Beijing Key Laboratory of Opto-electronic Functional Materials & Micro-nano Devices, Renmin University of China, Beijing 100872, China and Key Laboratory of Quantum State Construction and Manipulation (Ministry of Education), Renmin University of China, Beijing 100872, China

Description

High temperature superconductivity was recently found in the bilayer nickelate La3Ni2O7 (La327), followed by the discovery of superconductivity in the trilayer La4Ni3O10 (La4310), under high pressure. Through studying the electronic correlation of La4310 with DFT+DMFT, and further comparing it with that of La327, we find that the eg orbitals of the outer-layer Ni cations in La4310 have a similar (but slightly weaker) electronic correlation to those in La327, in which the electrons behave as a non-Fermi liquid with Hund correlation and linear-in-temperature scattering rate. Our results suggest that the experimentally observed "strange metal" behavior may be explained by the Hund spin correlation featuring high spin states and spin-orbital separation. In contrast, the electrons in the inner-layer Ni cations in La4310 behave as a Fermi liquid. The weaker electronic correlation in La4310 is attributed to more hole doping, which may explain its lower superconducting transition temperature.

Additional details

Identifiers

DOI
10.1103/PhysRevB.109.165140;
arXiv
arXiv:2402.02581;
Crossref Funder ID
10.13039/501100001809;

Publishing Information

Journal Title
Physical Review B
Journal Volume
109
Journal Issue
16
Journal Page Range
8 pgs.
ISSN
1550-235X

Optional Information

Copyright
©2024 American Physical Society
Contract/Grant/Project number
11934020
Notes
Contact Email: rqhe@ruc.edu.cn; Contact Email: zlu@ruc.edu.cn; Record automatically processed
Funding organization
National Natural Science Foundation of China