Non-Fermi liquid and Hund correlation in under high pressure
- 1. Department of Physics and Beijing Key Laboratory of Opto-electronic Functional Materials & Micro-nano Devices, Renmin University of China, Beijing 100872, China and Key Laboratory of Quantum State Construction and Manipulation (Ministry of Education), Renmin University of China, Beijing 100872, China
Description
High temperature superconductivity was recently found in the bilayer nickelate (La327), followed by the discovery of superconductivity in the trilayer (La4310), under high pressure. Through studying the electronic correlation of La4310 with , and further comparing it with that of La327, we find that the orbitals of the outer-layer Ni cations in La4310 have a similar (but slightly weaker) electronic correlation to those in La327, in which the electrons behave as a non-Fermi liquid with Hund correlation and linear-in-temperature scattering rate. Our results suggest that the experimentally observed "strange metal" behavior may be explained by the Hund spin correlation featuring high spin states and spin-orbital separation. In contrast, the electrons in the inner-layer Ni cations in La4310 behave as a Fermi liquid. The weaker electronic correlation in La4310 is attributed to more hole doping, which may explain its lower superconducting transition temperature.
Additional details
Identifiers
- DOI
- 10.1103/PhysRevB.109.165140;
- arXiv
- arXiv:2402.02581;
- Crossref Funder ID
- 10.13039/501100001809;
Publishing Information
- Journal Title
- Physical Review B
- Journal Volume
- 109
- Journal Issue
- 16
- Journal Page Range
- 8 pgs.
- ISSN
- 1550-235X
INIS
- Country of Publication
- United States
- Country of Input or Organization
- International Atomic Energy Agency (IAEA)
- Subject category
- S75: CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND SUPERFLUIDITY;
- Descriptors DEI
- CATIONS; COMPARATIVE EVALUATIONS; CORRELATIONS; ELECTRONS; FERMI GAS; FERMI LEVEL; HIGH SPIN STATES; HOLES; L-S COUPLING; LANTHANUM COMPOUNDS; LANTHANUM OXIDES; LAYERS; SCATTERING; SPIN; SUPERCONDUCTIVITY; TRANSITION TEMPERATURE
- Descriptors DEC
- ANGULAR MOMENTUM; CHALCOGENIDES; CHARGED PARTICLES; COUPLING; ELECTRIC CONDUCTIVITY; ELECTRICAL PROPERTIES; ELEMENTARY PARTICLES; ENERGY LEVELS; EVALUATION; FERMIONS; INTERMEDIATE COUPLING; IONS; LANTHANUM COMPOUNDS; LEPTONS; OXIDES; OXYGEN COMPOUNDS; PARTICLE PROPERTIES; PHYSICAL PROPERTIES; RARE EARTH COMPOUNDS; THERMODYNAMIC PROPERTIES
Optional Information
- Copyright
- ©2024 American Physical Society
- Contract/Grant/Project number
- 11934020
- Notes
- Contact Email: rqhe@ruc.edu.cn; Contact Email: zlu@ruc.edu.cn; Record automatically processed
- Funding organization
- National Natural Science Foundation of China