Published June 28, 2015
| Version v1
Journal article
Observation of low-energy electrons in the photoelectron energy distribution from strong-field ionization of naphthalene by circularly polarized pulses
- 1. Max Planck Institute for the Physics of Complex Systems, Nöthnitzer Strasse 38, D-01187 Dresden (Germany)
- 2. Department of Chemistry, Aarhus University, DK-8000 Aarhus C (Denmark)
- 3. Department of Physics and Astronomy, Aarhus University, DK-8000 Aarhus C (Denmark)
Description
In a joint experimental and theoretical study we reveal the presence of low-energy photoelectrons created by strong circularly polarized laser pulses for both 3D aligned and randomly oriented naphthalene molecules. The analysis within a semiclassical model highlights the essential role of the induced dipole of the molecular cation in the creation of these low-energy electrons. The detailed comparison of experiment and theory points to significant modification of the molecular orbital nodal planes in strong fields. (fast track communication)
Availability note (English)
Available from http://dx.doi.org/10.1088/0953-4075/48/12/121001Additional details
Identifiers
Publishing Information
- Journal Title
- Journal of Physics. B, Atomic, Molecular and Optical Physics
- Journal Volume
- 48
- Journal Issue
- 12
- Journal Page Range
- [6 p.]
- ISSN
- 0953-4075
- CODEN
- JPAPEH
INIS
- Country of Publication
- United Kingdom
- Country of Input or Organization
- International Atomic Energy Agency (IAEA)
- INIS RN
- 47103641
- Subject category
- S74: ATOMIC AND MOLECULAR PHYSICS;
- Descriptors DEI
- CATIONS; COMPARATIVE EVALUATIONS; DIPOLES; ELECTRONS; ENERGY SPECTRA; IONIZATION; LASER RADIATION; MODIFICATIONS; MOLECULAR ORBITAL METHOD; MOLECULES; NAPHTHALENE; PARTICLE TRACKS; PULSES; RANDOMNESS; SEMICLASSICAL APPROXIMATION
- Descriptors DEC
- APPROXIMATIONS; AROMATICS; CALCULATION METHODS; CHARGED PARTICLES; CONDENSED AROMATICS; ELECTROMAGNETIC RADIATION; ELEMENTARY PARTICLES; EVALUATION; FERMIONS; HYDROCARBONS; IONS; LEPTONS; MULTIPOLES; ORGANIC COMPOUNDS; RADIATIONS; SPECTRA