Published October 2017 | Version v1
Journal article

Delayed fission and multifragmentation in sub-keV C60 – Au(001) collisions via molecular dynamics simulations: Mass distributions and activated statistical decay

  • 1. Schulich Faculty of Chemistry, Technion – Israel Institute of Technology, 3200008 (Israel)

Description

We have recently observed, both experimentally and computationally, the phenomenon of postcollision multifragmentation in sub-keV surface collisions of a C60 projectile. Namely, delayed multiparticle breakup of a strongly impact deformed and vibrationally excited large cluster collider into several large fragments, after leaving the surface. Molecular dynamics simulations with extensive statistics revealed a nearly simultaneous event, within a sub-psec time window. Here we study, computationally, additional essential aspects of this new delayed collisional fragmentation which were not addressed before. Specifically, we study here the delayed (binary) fission channel for different impact energies both by calculating mass distributions over all fission events and by calculating and analyzing lifetime distributions of the scattered projectile. We observe an asymmetric fission resulting in a most probable fission channel and we find an activated exponential (statistical) decay. Finally, we also calculate and discuss the fragment mass distribution in (triple) multifragmentation over different time windows, in terms of most abundant fragments.

Availability note (English)

Available from http://dx.doi.org/10.1016/j.nimb.2017.05.060

Additional details

Identifiers

DOI
10.1016/j.nimb.2017.05.060;
PII
S0168583X17306584;

Publishing Information

Journal Title
Nuclear Instruments and Methods in Physics Research. Section B, Beam Interactions with Materials and Atoms
Journal Volume
409
Journal Page Range
p. 229-234
ISSN
0168-583X
CODEN
NIMBEU

Conference

Title
20. international conference on ion beam modification of materials
Acronym
IBMM 2016
Dates
30 Oct - 4 Nov 2016
Place
Wellington (New Zealand)

INIS

Country of Publication
Netherlands
Country of Input or Organization
International Atomic Energy Agency (IAEA)
INIS RN
51066082
Subject category
S73: NUCLEAR PHYSICS AND RADIATION PHYSICS; S75: CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND SUPERFLUIDITY;
Resource subtype / Literary indicator
Conference
Descriptors DEI
BINARY FISSION; COLLISIONS; DECAY; FRAGMENTATION; ION BEAMS; MASS DISTRIBUTION; MOLECULAR DYNAMICS METHOD; MOLECULAR IONS; SIMULATION; STATISTICS; SURFACES
Descriptors DEC
BEAMS; CALCULATION METHODS; CHARGED PARTICLES; DISTRIBUTION; FISSION; IONS; MATHEMATICS; NUCLEAR REACTIONS; SPATIAL DISTRIBUTION

Optional Information

Copyright
Copyright (c) 2017 Elsevier B.V. All rights reserved.