Published March 2007 | Version v1
Journal article

Magnetic dynamics of the spin-glass system PrAu2Si2: An inelastic neutron scattering study

  • 1. Materials Science Division, Argonne National Laboratory, Argonne, Illinois 60439 (United States) and ISIS Facility, Rutherford Appleton Laboratory, Chilton, Oxfordshire OX11 0QX (United Kingdom)
  • 2. Materials Science Division, Argonne National Laboratory, Argonne, Illinois 60439 (United States)
  • 3. Physics Departament, Southampton University, Southampton SO17 1BJ (United Kingdom)
  • 4. ISIS Facility, Rutherford Appleton Laboratory, Chilton, Oxfordshire OX11 0QX (United Kingdom)
  • 5. Institut Laue-Langevin, BP156, 38042 Grenoble Cedex 9 (France)

Description

In order to understand the origin of the spin glass ground state in the stoichiometric compound PrAu2Si2, we have performed inelastic neutron scattering measurements of the crystal field (CF) excitation spectrum. The 4f ground state is a Γ 4 singlet and the first excited level is a Γ 5(2) doublet at 0.72 meV. We compare the CF potential with other isostructural compounds to determine what features of the CF splittings are essential in producing spin glass freezing in a structurally ordered compound

Additional details

Identifiers

DOI
10.1016/j.jmmm.2006.10.452;
PII
S0304-8853(06)01659-3;

Publishing Information

Journal Title
Journal of Magnetism and Magnetic Materials
Journal Volume
310
Journal Issue
2
Journal Page Range
p. 1535-1536
ISSN
0304-8853
CODEN
JMMMDC

Conference

Title
17. international conference on magnetism
Dates
20-25 Aug 2006
Place
Kyoto (Japan)

INIS

Country of Publication
Netherlands
Country of Input or Organization
International Atomic Energy Agency (IAEA)
INIS RN
39029794
Subject category
S36: MATERIALS SCIENCE;
Resource subtype / Literary indicator
Conference
Descriptors DEI
CRYSTAL FIELD; EXCITED STATES; GOLD COMPOUNDS; GROUND STATES; INELASTIC SCATTERING; NEUTRON DIFFRACTION; PRASEODYMIUM COMPOUNDS; SILICIDES; SPECTRA; SPIN GLASS STATE
Descriptors DEC
COHERENT SCATTERING; DIFFRACTION; ENERGY LEVELS; RARE EARTH COMPOUNDS; SCATTERING; SILICON COMPOUNDS; TRANSITION ELEMENT COMPOUNDS

Optional Information

Copyright
Copyright (c) 2006 Elsevier Science B.V., Amsterdam, The Netherlands, All rights reserved.