Published March 12, 2010 | Version v1
Journal article

Cholesterol-Phospholipid Interactions: New Insights from Surface X-Ray Scattering Data

  • 1. Center for Molecular Study of Condensed Soft Matter (muCoSM), and Division of Physics, BCPS Department, Illinois Institute of Technology, Chicago, Illinois 60616 (United States)
  • 2. Advanced Photon Source, Argonne National Laboratories, Argonne, Illinois 60439 (United States)

Description

We report a structural study of cholesterol-DPPC (1,2-dipalmitoyl-sn-glycero-3-phophocholine) monolayers using x-ray reflectivity and grazing incidence x-ray diffraction. Reflectivity reveals that the vertical position of cholesterol relative to phospholipids strongly depends on its mole fraction (χCHOL). Moreover, we find that at a broad range of χCHOL cholesterol and DPPC form alloylike mixed domains of short-range order and the same stoichiometry as that of the film. Based on the data presented, we propose a new model of cholesterol-phospholipid organization in mixed monolayers.

Additional details

Publishing Information

Journal Title
Physical Review Letters
Journal Volume
104
Journal Issue
10
Journal Page Range
p. 108101-108101.4
ISSN
0031-9007
CODEN
PRLTAO

Optional Information

Notes
(c) 2010 The American Physical Society