Published December 2004 | Version v1
Journal article

Phase transition behaviour in the A-site deficient perovskite oxide La1/3NbO3

  • 1. Centre for Structural Chemistry and Biology, School of Chemistry, University of Sydney, F11, Sydney, New South Wales 2006 (Australia)
  • 2. School of Physics, The University of Sydney, Sydney, New South Wales 2006 (Australia)
  • 3. Australian Nuclear Science and Technology Organisation, Private Mail Bag 1, Menai, New South Wales 2234 (Australia)
  • 4. Department of Environmental Sciences, Faculty of Science, Osaka Women's University, Daisen-cho 2-1, Sakai, Osaka 590-0035 (Japan)
  • 5. Japan Synchrotron Radiation Research Institute, 1-1-1 Kouto, Mikazuki-cho, Sayo-gun, Hyogo 679-5198 (Japan)

Description

The crystal structure of the layered perovskite La1/3NbO3 has been studied between room temperature and 500oC using synchrotron X-ray powder diffraction methods. The structure shows ordering of the La cations at all temperatures. At room temperature La1/3NbO3 is orthorhombic with the NbO6 octahedra showing out-of-phase tilting about the a-axis. This tilting diminishes as the temperature increases, so that above 200oC the structure is tetragonal. The transition to the tetragonal structure is found to be continuous and analysis of the spontaneous strains shows it to be tricritical in nature

Additional details

Identifiers

DOI
10.1016/j.jssc.2004.08.047;
PII
S0022-4596(04)00472-4;

Publishing Information

Journal Title
Journal of Solid State Chemistry
Journal Volume
177
Journal Issue
12
Journal Page Range
p. 4552-4556
ISSN
0022-4596
CODEN
JSSCBI

Optional Information

Copyright
Copyright (c) 2004 Elsevier Science B.V., Amsterdam, The Netherlands, All rights reserved.