Screened hydrogen model of excitons in semiconducting nanoribbons
- 1. Departamento de Ciencias, Universidad Privada del Norte, Lima 15434, Peru
- 2. Instituto de Física Teórica, Universidade Estadual Paulista (UNESP), Rua Dr. Bento T. Ferraz, 271, São Paulo, SP 01140-070, Brazil
Description
The optical response of quasi-one-dimensional systems is often dominated by tightly bound excitons that significantly influence their basic electronic properties. Despite their importance for device performance, accurately predicting their excitonic effects typically requires computationally demanding many-body approaches. Here, we present a simplified model to describe the static macroscopic dielectric function, which depends only on the width of the quasi-one-dimensional system and its polarizability per unit length. We show that at certain interaction distances, the screened Coulomb potential is greater than its bare counterpart, which results from the enhanced repulsive electron-electron interactions. As a test case, we study 14 different nanoribbons, 12 of them armchair graphene nanoribbons of different families. Initially, we devised a simplified equation to estimate the exciton binding energy and extension that provides results comparable to those from the full Bethe-Salpeter equation, albeit for a specific nanoribbon family. Then, we used our proposed screening potential to solve the 1D Wannier-Mott equation, which turns out to be a broad approach that is able to predict binding energies that match quite well the ones obtained with the Bethe-Salpeter equation, irrespective of the nanoribbon family.
Additional details
Identifiers
- DOI
- 10.1103/PhysRevB.109.165425;
- Crossref Funder ID
- 10.13039/501100001807; 10.13039/501100003593;
Publishing Information
- Journal Title
- Physical Review B
- Journal Volume
- 109
- Journal Issue
- 16
- Journal Page Range
- 8 pgs.
- ISSN
- 1550-235X
INIS
- Country of Publication
- United States
- Country of Input or Organization
- International Atomic Energy Agency (IAEA)
- Subject category
- S77: NANOSCIENCE AND NANOTECHNOLOGY; S75: CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND SUPERFLUIDITY;
- Descriptors DEI
- BETHE-SALPETER EQUATION; BINDING ENERGY; COULOMB FIELD; DIELECTRIC MATERIALS; DIELECTRIC PROPERTIES; DISTANCE; EXCITONS; FUNCTIONS; GRAPHENE; HYDROGEN; INTERACTIONS; LENGTH; MANY-BODY PROBLEM; NANOSTRUCTURES; POTENTIALS
- Descriptors DEC
- CARBON; DIMENSIONS; ELECTRIC FIELDS; ELECTRICAL PROPERTIES; ELEMENTS; ENERGY; EQUATIONS; MATERIALS; NONMETALS; PHYSICAL PROPERTIES; QUASI PARTICLES
Optional Information
- Copyright
- ©2024 American Physical Society
- Contract/Grant/Project number
- 2016/01343-7; 2017/02317-2; 2021/14335-0; 408038/2022-5; 307710/2019-0
- Notes
- Record automatically processed
- Funding organization
- Fundação de Amparo à Pesquisa do Estado de São Paulo; Conselho Nacional de Desenvolvimento Científico e Tecnológico