Published October 1985 | Version v1
Journal article

Thermal, photo- and radiation stability of hydroxotetranitronitrosoruthenates

  • 1. Moskovskij Inst. Tonkoj Khimicheskoj Tekhnologii (USSR)

Description

Thermal, photo- and radiation stability of hydroxotetranitronitrosoruthenates M[Ru(NO)(NO2)4OH]xnH2O, where M-Sr, Ba, Zn, Pb, Na, Ag are studied. The decomposition of the compounds in vacuum, as well as their thermal decomposition in the air, depends on the second sphere cation, with the water and NO molecules, being the main gaseous products. Two temperature maxima for the NO-group removal are measured. In the process of gamma - irradiation with a dose of 5-6 M rad (77 K) of the compound polycrystal samples the tabilization of NO2 and NO22- radicals was observed. It is shown, that during photolysis either the formation of trivalent ruthenium complexes very likely at the expense of solvent molecule substitution for nitrosogroup, or of paramagnetic compound, in which uncoupled electron is localized mainly on a nitrosogroup (g sub(tr) approximately equal to 2, g sub(long)=1.916, Asub(tr)sup(N) approximately equal to 30 Oe), take place depending on photolysis conditions

Additional details

Additional titles

Original title (Russian)
Термическая, фото- и радиационня устойчивост' гидроксотетранитронитрозорутенатов

Publishing Information

Journal Title
Zh. Neorg. Khim.
Journal Volume
30
Journal Issue
10
Series
Zh. Neorg. Khim.
Journal Page Range
2605-2609
ISSN
0044-457X
CODEN
ZNOKA

Optional Information

Notes
For English translation see the journal Russian Journal of Inorganic Chemistry (UK).