Published February 26, 2024 | Version v1
Journal article

Heavy fermion related behaviors and the effects from nonmagnetic atom vacancies in the 5f-electron based antiferromagnet UAs2

  • 1. Science and Technology on Surface Physics and Chemistry Laboratory, Mianyang 621908, China

Description

Recent studies on the electronic structures of the 5f-electron based antiferromagnetic compounds, i.e., uranium dipnictides, have aroused widespread interest in the complex interplay among different channels of interactions, such as Kondo entanglement and antiferromagnetic ordering. Here, we use scanning tunneling microscopy/spectroscopy to explore the complex low-energy excitations in the 5f-electron based antiferromagnet UAs2. The crystal-field excitations are revealed as peaks above the Fermi level in the dI/dV spectra. Temperature-dependent spectroscopic measurements find that Kondo resonance and antiferromagnetic order are manifested as two peaks below the Fermi level, demonstrating that Kondo coherence can be undisturbedly established in the antiferromagnetic phase. The crystal-field excitations, Kondo resonance, and antiferromagnetic state are all locally altered by the presence of As-atom vacancies at the atomic scale and these phenomena prove that the nonmagnetic atom vacancy has a strong influence on low-energy excitations in heavy fermion compounds.

Additional details

Identifiers

DOI
10.1103/PhysRevB.109.075158;
Crossref Funder ID
10.13039/501100012166; 10.13039/501100001809;

Publishing Information

Journal Title
Physical Review B
Journal Volume
109
Journal Issue
7
Journal Page Range
9 pgs.
ISSN
1550-235X

Optional Information

Copyright
©2024 American Physical Society
Contract/Grant/Project number
2021YFA1601101; 2022YFA1402201; U23A20580; 12004349; 11904335; 12122409; 11974319; 21903074; 11904334; 11774320
Notes
Contact Email: liuqin493@163.com; Contact Email: sytan4444@163.com; Contact Email: lxcydbj@163.com; Record automatically processed
Funding organization
National Key Research and Development Program of China; National Natural Science Foundation of China