Published March 2011 | Version v1
Journal article

Li Ion Diffusivity and Improved Electrochemical Performances of the Carbon Coated LiFePO4

  • 1. Korea Institute of Science and Technology, Seoul (Korea, Republic of)
  • 2. Korea University, Seoul (Korea, Republic of)

Description

This study examines the effects of a carbon coating on the electrochemical performances of LiFePO4. The results show that the capacity of bare LiFePO4 decreased sharply, whereas the LiFePO4/C shows a well maintained initial capacity. The Li ion diffusivity of the bare and carbon coated LiFePO4 is calculated using cyclic voltammetry (CV) to determine the correlation between the electrochemical performance of LiFePO4 and Li diffusion. The diffusion constants for LiFePO4 and LiFePO4/C measured from CV are 6.56 x 10-16 and 2.48 x 10-15 cm2 s-1, respectively, indicating considerable increases in diffusivity after modifications. The Li ion diffusivity (DLi) values as a function of the lithium content in the cathode are estimated by electrochemical impedance spectroscopy (EIS). The effects of the carbon coating as well as the mechanisms for the improved electrochemical performances after modification are discussed based on the diffusivity data

Additional details

Publishing Information

Journal Title
Bulletin of the Korean Chemical Society
Journal Volume
32
Journal Issue
3
Series
28 refs, 8 figs, 2 tabs
Journal Page Range
p. 836-840
ISSN
0253-2964

INIS

Country of Publication
Korea, Republic of
Country of Input or Organization
Korea, Republic of
INIS RN
47121466
Subject category
S37: INORGANIC, ORGANIC, PHYSICAL AND ANALYTICAL CHEMISTRY;
Descriptors DEI
DIFFUSION; ELECTROCHEMISTRY; LITHIUM IONS; MAINTENANCE; MODIFICATIONS; PERFORMANCE
Descriptors DEC
CHARGED PARTICLES; CHEMISTRY; IONS