Transmission measurements and resonance parameter analysis for Mo-98 and Mo-100

Highlights: • High-resolution time-of-flight neutron transmission measurements on enriched metallic samples of Mo-98 and Mo-100. • The Bayesian R-Matrix code SAMMY 8.0 was used to shape-fit the data and extract resonance parameters from the data. • The results represent a refinement of those given in the current evaluation due to improvements in experimental resolution. - Abstract: Molybdenum can exist in many nuclear reactor components, including fuel, cladding, or as a high yield fission product. As a result, accurate isotopic nuclear data for molybdenum are important for reactor simulation. To this end, high-resolution time-of-flight neutron transmission measurements on highly enriched isotopic metallic samples of Mo-98 and Mo-100 were performed and data were reduced to transmission in the resolved resonance region from 10 eV to 53 keV for Mo-98 and 10 eV to 26.5 keV for Mo-100. Measurements were taken with Li-6 glass transmission detectors at 31 m and 100 m flight paths. The Bayesian R-matrix code SAMMY 8.0 was used to shape-fit the data and to extract resonance parameters from the transmission spectra. The newly fitted resonance parameters were compared with those given in ENDF/B-VII.1. The results represent a refinement of those given in the current evaluation due to the improvement in the experimental resolution in these measurements. The comparison included analysis of level statistics. The resonance parameters for Mo-98 show many differences with the current evaluations. The results of the analysis indicated missing levels in Mo-98 starting at 10 keV, which implies an inability to resolve all resonances at higher energies. The resonance parameters for Mo-100 agree well with the current evaluation. Level statistics analysis indicates there are few missing levels up to 26.5 keV.