Development of a reference spent fuel library of 17x17 PWR fuel assemblies

One of the most common ways to investigate new Non- Destructive Assays (NDA) for the spent fuel assemblies are Monte Carlo simulations. In order to build realistic models the user must define in an accurate way the material compositions and the source terms in the system. This information can be obtained using burnup codes such as ORIGEN-ARP and ALEPH2.2, developed at SCK•CEN. These software applications allow the user to select the irradiation history of the fuel assembly and to calculate the corresponding isotopic composition and neutron/gamma emissions as a function of time. In the framework of the development of an innovative NDA for spent fuel verifications, SCK•CEN built an extensive fuel library for 17x17 PWR assemblies, using both ORIGENARP and ALEPH2.2. The parameters considered in the calculations were initial enrichment, discharge burnup, and cooling time. The combination of these variables allows to obtain more than 1500 test cases. Considering the broad range of the parameters, the fuel library can be used for other purposes apart from spent fuel verifications, for instance for the direct disposal in geological repositories. In addition to the isotopic composition of the spent fuel, the neutron and photon emissions were also calculated and compared between the two codes. The comparison of the isotopic composition showed a good agreement between the codes for most of the relevant isotopes in the spent fuel. However, specific isotopes as well as neutron and gamma spectra still need to be investigated in detail.