Distribution of natural and anthropogenic radionuclides in soil and beach sand samples of Kalpakkam (India) using hyper pure germanium (HPGe) gamma ray spectrometry

Pre-operational survey at Kalpakkam coast, indicated elevated gamma background radiation levels in the range of 100-4000 nGy h-1 over the large tracts of the coastal sands due to the presence of pockets of monazite mineral in beach sands. In view of the prevalence of monazite, a systematic gamma spectrometric study of distribution of natural radionuclides in soil and beach sand samples collected from the terrestrial and coastal environment of Kalpakkam was performed and concentrations of primordial radionuclides such as 238U, 232Th and 40K and anthropogenic radionuclide 137Cs were determined. The concentrations of 238U, 232Th and 40K in soil samples were 5-71, 15-776 and 200-854 Bq kg-1 dry, respectively. In beach sand samples, 238U, 232Th and 40K contents varied in the range of 36-258, 352-3872 and 324-405 Bq kg-1 dry, respectively. The total absorbed gamma dose rate in air due to the presence of 238U, 232Th and 40K in Kalpakkam soil samples varied between 24 and 556 nGy h-1 with a mean of 103 nGy h-1. The contribution to the total absorbed gamma dose rate in air in the decreasing order was due to the presence of 232Th (76.4%), followed by 40K (16.9%) and 238U (6.7%) in Kalpakkam soils. However, in beach areas of Kalpakkam, the presence of 232Th in beach sand contributed maximum (94.0%) to the total absorbed gamma dose rate in air followed by 238U (4.7%) and minimum contribution was by 40K (1.3%). 137Cs in Kalpakkam soils ranged from ≤1.0 to 2.8 Bq kg-1 dry, which was 1-3 order of magnitude less than the concentration of primordial radionuclides in soil