Published May 20, 2024 | Version v1
Journal article

Microscopic theory for nonequilibrium correlation functions in dense active fluids

  • 1. Department of Applied Physics, Eindhoven University of Technology, P.O. Box 513, 5600MB Eindhoven, The Netherlands
  • 2. Institute for Complex Molecular Systems, Eindhoven University of Technology, P.O. Box 513, 5600MB Eindhoven, The Netherlands
  • 3. Département de Physique de l'Ecole Normale Supérieure, ENS, Université PSL, 24 rue Lhomond, 75230 Paris Cedex 05, France
  • 4. Institut für Materialphysik im Weltraum, Deutsches Zentrum für Luft- und Raumfahrt, 51170 Köln, Germany
  • 5. Department of Physics, Heinrich-Heine Universität Düsseldorf, Universitätsstraße 1, 40225 Düsseldorf, Germany

Description

One of the key hallmarks of dense active matter in the liquid, supercooled, and solid phases is the so-called equal-time velocity correlations. Crucially, these correlations can emerge spontaneously, i.e., they require no explicit alignment interactions, and therefore represent a generic feature of dense active matter. This indicates that for a meaningful comparison or possible mapping between active and passive liquids one not only needs to understand their structural properties, but also the impact of these velocity correlations. This has already prompted several simulation and theoretical studies, though they are mostly focused on athermal systems and thus overlook the effect of translational diffusion. Here, we present a fully microscopic method to calculate nonequilibrium correlations in two-dimensional systems of thermal active Brownian particles (ABPs). We use the integration through transients formalism together with (active) mode-coupling theory and analytically calculate qualitatively consistent static structure factors and active velocity correlations. We complement our theoretical results with simulations of both thermal and athermal ABPs which exemplify the disruptive role that thermal noise has on velocity correlations.

Additional details

Identifiers

DOI
10.1103/PhysRevE.109.054605;
arXiv
arXiv:2310.14812;
Crossref Funder ID
10.13039/501100003246; 10.13039/100015400;

Publishing Information

Journal Title
Physical Review E
Journal Volume
109
Journal Issue
5
Journal Page Range
11 pgs.
ISSN
1089-3787

Optional Information

Copyright
©2024 American Physical Society
Contract/Grant/Project number
2022-1-FR01-KA131-HED-000054547
Notes
These authors contributed equally to this work.; Contact Email: l.m.c.janssen@tue.nl; Record automatically processed
Funding organization
Nederlandse Organisatie voor Wetenschappelijk Onderzoek; Fonds Erasme