Study of K, L vacancies production mechanisms by X spectrometry in the interaction induced by a few MeV/A charged particles
Description
The analysis of different mechanisms producing electronic inner shell vacancies in ion atom collisions at a few MeV/A charged is presented. The mutual influence of nuclear and atomic excitation in the ionization probability has been discussed. The 106Cd(p,p')106Cd reaction (Ep=10 MeV) has been particularly investigated from this point. The investigation is followed up by the description of the theoretical and experimental methods which permit the determination of the total and/or differential X rays production cross section for different interaction. The gold sub-shell L1, L2, L3 ionization probability has been studied in the Au(H+,H+)Au reaction at Ep=1 MeV. In the second part of the manuscript we investigate in detail the influence of the charge exchange process on inner shell vacancy production. The N2, Ar, Kr targets have been produced by a system jet gas and bombarded by 0.8<=Ep<=3.5 MeV proton and 28Si14+ ions at E=125 MeV. The cross section for the capture of an electron in K shell, L shell and total charge exchange have been measured and compared to the CDW theory (Continuum Distorted Wave). In the CDW validity domain the experimental and theoretical results are a good agreement. In the collisions induced by H+, ionization is found to be the main excitation process. On the contrary, in collisions induced by 28Si14+ charge exchange is dominant compared to ionization
Availability note (English)
MF available from INIS under the Report Number.Abstract (French)
Les differents mecanismes pouvant conduire a la creation de lacunes en couches electroniques profondes d'un atome lors des collisions induites par des particules chargees de quelques MeV/A sont decrits. L'influence mutuelle des processus nucleaire et atomique est discutee dans la determination de la probabilite d'ionisation. La reaction 106Cd(p,p)106Cd (Ep=10 MeV) a ete de ce point de vue particulierement etudiee. Les methodes theoriques et experimentales permettant la determination de la section efficace totale et/ou differentielle de production de raies X pour diverses interactions sont analysees. Les probabilites d'ionisation des sous-couches L1, L2 et L3 de l'or ont ete etudiees dans la reaction Au(H+,H+)Au a Ep=1 MeV. La deuxieme partie de l'etude est consacree aux processus d'echange de charge. Les cibles N2, Ar, Kr ont ete produites au moyen d'un jet gazeux et ont ete irradiees par des protons 0.8<=Ep<=3.5 MeV et par des ions 28Si14+ a E=125 MeV. Les sections efficaces de capture totale et de capture en couche K et L ont ete mesurees et confrontees a la theorie CDW (Continuum Distorted Wave). Dans le domaine de validite de l'approximation CDW l'accord est correct en ce qui concerne la section efficace de capture totale. Il est montre que dans les deux situations abordees les deux processus, ionisation et echange de charge, jouent des roles diametralement opposes; pour la reaction par protons c'est l'ionisation qui est determinante par contre pour les reactions induites par les 28Si14+ c'est l'echange de charge qui est preponderantFiles
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Additional details
Additional titles
- Original title (French)
- Etude par spectrometrie X des mecanismes de production de lacunes K, L lors des interactions induites par des particules chargees de quelques MeV/A
Publishing Information
- Imprint Pagination
- 206 p.
- Report number
- CENBG--8108
INIS
- Country of Publication
- France
- Country of Input or Organization
- France
- INIS RN
- 14729760
- Subject category
- S74: ATOMIC AND MOLECULAR PHYSICS;
- Resource subtype / Literary indicator
- Numerical Data, Thesis
- Descriptors DEI
- CADMIUM 106 TARGET; CHARGE EXCHANGE; COULOMB IONIZATION; ELASTIC SCATTERING; EXPERIMENTAL DATA; INNER-SHELL IONIZATION; ION-ATOM COLLISIONS; K SHELL; L SHELL; PROBABILITY; PROTON REACTIONS; X-RAY SPECTROSCOPY
- Descriptors DEC
- ATOM COLLISIONS; BARYON REACTIONS; COLLISIONS; DATA; ELECTRONIC STRUCTURE; HADRON REACTIONS; INFORMATION; ION COLLISIONS; IONIZATION; NUCLEAR REACTIONS; NUCLEON REACTIONS; NUMERICAL DATA; SCATTERING; SPECTROSCOPY; TARGETS