Published July 2002 | Version v1
Journal article

Crystal growth of thermoelectric material NaxCoO2-δ by a flux method

  • 1. Osaka University, Department of Electrical Engineering, Suita, Osaka (Japan)
  • 2. National Institute of Advanced Industrial Science and Technology, Ikeda, Osaka (Japan)

Description

NaxCoO2-δ (0.5≤x≤1) crystals were grown by a flux method. The largest NaxCoO2-δ crystal size was 10x10x0.5 mm3, and the crystal phase depended on the composition of the flux. Crystals grown from a flux of NaCl mixed with Na2CO3 and B2O3 and crystals grown from a flux of Na2CO3 mixed with B2O3 were identified as Na0.6CoO2-δ (γ phase) and Na0.9CoO2-δ (α phase), respectively. The structures and compositions of these crystal growths were determined with a power X-ray diffraction device and an energy dispersive X-ray spectrometer, respectively. The in-plane thermoelectric power values of these two types of crystal increased with temperature and reached 96 μV/K and 87 μV/K at 450K, respectively. (author)

Additional details

Publishing Information

Journal Title
Japanese Journal of Applied Physics. Part 2, Letters
Journal Volume
41
Journal Issue
7A
Journal Page Range
p. L777-L779
ISSN
0021-4922

Optional Information

Notes
8 refs., 4 figs.