Strong-field approximation for Coulomb explosion of H2+ and D2+ by short intense laser pulses
Creators
- 1. Lundbeck Foundation Theoretical Center for Quantum System Research, Department of Physics and Astronomy, University of Aarhus, 8000 Aarhus C (Denmark)
- 2. Centre for Theoretical Atomic Molecular and Optical Physics, School of Mathematics and Physics, Queen's University Belfast, Belfast BT7 1NN (United Kingdom)
Description
We present a simple quantum mechanical model to describe Coulomb explosion of H2+ and D2+ by short, intense infrared laser pulses. The model is based on the length gauge version of the molecular strong-field approximation and is valid when the process of dissociation prior to ionization is negligible. The results are compared with recent experimental data for the proton kinetic energy spectrum [Th. Ergler et al., Phys. Rev. Lett. 95, 093001 (2005); D. S. Murphy et al., J. Phys. B 40, S359 (2007)]. Using a Franck-Condon distribution over initial vibrational states, the theory reproduces the overall shape of the spectrum with only a small overestimation of slow protons. The agreement between theory and experiment can be made perfect by using a non-Frank-Condon initial distribution characteristic for H2+ (D2+) targets produced by strong-field ionization of H2 (D2). For comparison, we also present results obtained by two different tunneling models for this process
Additional details
Identifiers
- DOI
- 10.1103/PhysRevA.76.033414;
- arXiv
- arXiv:0704.2479v1;
Publishing Information
- Journal Title
- Physical Review. A
- Journal Volume
- 76
- Journal Issue
- 3
- Journal Page Range
- p. 033414-033414.8
- ISSN
- 1050-2947
- CODEN
- PLRAAN
INIS
- Country of Publication
- United States
- Country of Input or Organization
- International Atomic Energy Agency (IAEA)
- INIS RN
- 39042345
- Subject category
- S74: ATOMIC AND MOLECULAR PHYSICS;
- Descriptors DEI
- APPROXIMATIONS; BEAMS; COMPARATIVE EVALUATIONS; DEUTERIUM; DEUTERIUM IONS; DISTRIBUTION; FRANCK-CONDON PRINCIPLE; HYDROGEN; HYDROGEN IONS 1 PLUS; INFRARED RADIATION; LASER RADIATION; MOLECULAR IONS; PHOTOIONIZATION; PHOTOLYSIS; PROTONS; PULSES; QUANTUM MECHANICS; SPECTRA; TUNNEL EFFECT; VIBRATIONAL STATES
- Descriptors DEC
- BARYONS; CALCULATION METHODS; CATIONS; CHARGED PARTICLES; CHEMICAL REACTIONS; DECOMPOSITION; ELECTROMAGNETIC RADIATION; ELEMENTARY PARTICLES; ELEMENTS; ENERGY LEVELS; EVALUATION; EXCITED STATES; FERMIONS; HADRONS; HYDROGEN IONS; HYDROGEN ISOTOPES; IONIZATION; IONS; ISOTOPES; LIGHT NUCLEI; MECHANICS; NONMETALS; NUCLEI; NUCLEONS; ODD-ODD NUCLEI; PHOTOCHEMICAL REACTIONS; RADIATIONS; STABLE ISOTOPES
Optional Information
- Notes
- (c) 2007 The American Physical Society