Published September 2007 | Version v1
Journal article

Strong-field approximation for Coulomb explosion of H2+ and D2+ by short intense laser pulses

  • 1. Lundbeck Foundation Theoretical Center for Quantum System Research, Department of Physics and Astronomy, University of Aarhus, 8000 Aarhus C (Denmark)
  • 2. Centre for Theoretical Atomic Molecular and Optical Physics, School of Mathematics and Physics, Queen's University Belfast, Belfast BT7 1NN (United Kingdom)

Description

We present a simple quantum mechanical model to describe Coulomb explosion of H2+ and D2+ by short, intense infrared laser pulses. The model is based on the length gauge version of the molecular strong-field approximation and is valid when the process of dissociation prior to ionization is negligible. The results are compared with recent experimental data for the proton kinetic energy spectrum [Th. Ergler et al., Phys. Rev. Lett. 95, 093001 (2005); D. S. Murphy et al., J. Phys. B 40, S359 (2007)]. Using a Franck-Condon distribution over initial vibrational states, the theory reproduces the overall shape of the spectrum with only a small overestimation of slow protons. The agreement between theory and experiment can be made perfect by using a non-Frank-Condon initial distribution characteristic for H2+ (D2+) targets produced by strong-field ionization of H2 (D2). For comparison, we also present results obtained by two different tunneling models for this process

Additional details

Publishing Information

Journal Title
Physical Review. A
Journal Volume
76
Journal Issue
3
Journal Page Range
p. 033414-033414.8
ISSN
1050-2947
CODEN
PLRAAN

Optional Information

Notes
(c) 2007 The American Physical Society