Influences of reprocessing separation efficiency on the fuel cycle performances for a Heavy Water moderated Molten Salt Reactor

Highlights: • Influences of reprocessing separation efficiency (RSE) on HWMSR fuel cycle performances are analyzed. • Lowering RSE would improve the breeding ratio but prolong the double time. • Radiotoxicity of lost heavy metal decreases with RSE and reprocessing cycle time (RCT). • An RCT of 60 days is recommended for HWMSR with the RSE of 99.9%. Reprocessing separation efficiency (RSE) is one important fuel cycle indicator which determines the loss of actinides left in the nuclear waste and the recovered actinides for reuse in the core, affecting the nuclear waste management, fuel utilization and other fuel cycle characteristics. By changing the reprocessing cycle time (RCT) from 10 days to 360 days, the impacts of RSE varying from 99.9% to 99.999% on the core actinides inventory evolution, breeding ratio (BR) and nuclear waste radiotoxicity were investigated for a Heavy Water moderated Molten Salt Reactor (HWMSR), which is a newly proposed molten salt reactor (MSR) that adopts heavy water rather than graphite as the moderator while employs the usual liquid fuel as in a traditional MSR. The obtained results demonstrate that the inventories of transuranic (TRU) and uranium except U-233 at equilibrium and their transition time to equilibrium both decreases as RSE declines due to their increased mass loss in reprocessing, which in turn brings down the parasitic neutron absorption in the core. Consequently, the U-233 inventory required for maintaining critical operation for a lower RSE drops. While the Th-232 inventory rises, since it is online refueled to maintain the total heavy metal (HM) content in the core constant to ensure the electrochemical stability of the fuel salt. As a result, BR is relatively improved as RSE decreases. But the increased U-233 production resulting from the improved BR could not compensate for the U-233 loss during reprocessing and leads to a longer doubling time for a lower RSE. The radiotoxicity of nuclear waste increases as RSE decreases since more actinides are lost to the nuclear waste. The above effects caused by RSE are mitigated as the RCT prolongs since the frequency for reprocessing the fuel salt of primary loop over a given period decreases, leading to a decrease of HM loss. For an RSE level of 99.9%, the shortest doubling time appears at the RCT of 30 days rather than 10 days because the mitigation of U-233 loss overwhelms the efficiency decrease of FPs removal and Pa-233 extraction. By balancing the Th-U breeding and radiotoxicity, an RCT of 60 days is recommended for HWMSR for the RSE of 99.9%.