Published 2012
| Version v1
Journal article
Effect of groundwater on the dissolution rate of the simulated nuclear waste glass SON68 under gamma irradiation
- 1. CEA, DEN, DTCD, SECM, F-30207 Bagnols Sur Ceze, (France)
- 2. INERIS, Parc Technologique Alata, BP2 F-60550 Verneuil en Halatte, (France)
- 3. Universite Lyon, Universite Lyon1, CNRS/ISA, UFR de Chimie Biochimie, 69622 Villeurbanne cedex, (France)
Description
The leaching behaviour of the inactive reference of the R7T7 glass is investigated here in a synthetic clayey groundwater solution, focusing on the effect of gamma irradiation on this residual alteration rate, under static conditions, at 90 degrees C. Results don't underline any significant effect of gamma irradiation on the residual alteration rate up to 5 kGy/h, compared to experiments performed out of irradiation in groundwater or in pure water. Moreover, the evolution of boron releases in groundwater versus time is similar whatever the dose rate. These observations are consistent with SEM characterizations. (authors)
Additional details
Identifiers
Publishing Information
- Journal Title
- Procedia Chemistry
- Journal Volume
- 7
- Journal Page Range
- p. 587-592
- ISSN
- 1876-6196
Conference
- Title
- International Conference on Nuclear Chemistry for Sustainable Fuel Cycles
- Acronym
- Atalante 2012
- Dates
- 2-7 Sep 2012
- Place
- Le Corum, Montpellier (France)
INIS
- Country of Publication
- France
- Country of Input or Organization
- France
- INIS RN
- 45077184
- Subject category
- S12: MANAGEMENT OF RADIOACTIVE WASTES, AND NON-RADIOACTIVE WASTES FROM NUCLEAR FACILITIES;
- Resource subtype / Literary indicator
- Conference
- Descriptors DEI
- AQUEOUS SOLUTIONS; BOROSILICATE GLASS; CHEMICAL REACTION KINETICS; CLAYS; GAMMA RADIATION; GROUND WATER; LEACHING; RADIOACTIVE WASTE DISPOSAL; RADIOLYSIS; UNDERGROUND STORAGE
- Descriptors DEC
- CHEMICAL RADIATION EFFECTS; CHEMICAL REACTIONS; DECOMPOSITION; DISPERSIONS; DISSOLUTION; ELECTROMAGNETIC RADIATION; GLASS; HOMOGENEOUS MIXTURES; HYDROGEN COMPOUNDS; IONIZING RADIATIONS; KINETICS; MANAGEMENT; MINERALS; MIXTURES; OXYGEN COMPOUNDS; RADIATION EFFECTS; RADIATIONS; RADIOACTIVE WASTE MANAGEMENT; REACTION KINETICS; SEPARATION PROCESSES; SILICATE MINERALS; SOLUTIONS; STORAGE; WASTE DISPOSAL; WASTE MANAGEMENT; WATER
Optional Information
- Notes
- 20 refs.