Published 2012 | Version v1
Journal article

Effect of groundwater on the dissolution rate of the simulated nuclear waste glass SON68 under gamma irradiation

  • 1. CEA, DEN, DTCD, SECM, F-30207 Bagnols Sur Ceze, (France)
  • 2. INERIS, Parc Technologique Alata, BP2 F-60550 Verneuil en Halatte, (France)
  • 3. Universite Lyon, Universite Lyon1, CNRS/ISA, UFR de Chimie Biochimie, 69622 Villeurbanne cedex, (France)

Description

The leaching behaviour of the inactive reference of the R7T7 glass is investigated here in a synthetic clayey groundwater solution, focusing on the effect of gamma irradiation on this residual alteration rate, under static conditions, at 90 degrees C. Results don't underline any significant effect of gamma irradiation on the residual alteration rate up to 5 kGy/h, compared to experiments performed out of irradiation in groundwater or in pure water. Moreover, the evolution of boron releases in groundwater versus time is similar whatever the dose rate. These observations are consistent with SEM characterizations. (authors)

Additional details

Identifiers

Publishing Information

Journal Title
Procedia Chemistry
Journal Volume
7
Journal Page Range
p. 587-592
ISSN
1876-6196

Conference

Title
International Conference on Nuclear Chemistry for Sustainable Fuel Cycles
Acronym
Atalante 2012
Dates
2-7 Sep 2012
Place
Le Corum, Montpellier (France)

Optional Information

Notes
20 refs.