Published October 2011 | Version v1
Journal article

Numerical studies of the interaction of an atomic sample with the electromagnetic field in two dimensions

  • 1. Department of Applied Sciences and Mathematics, Arizona State University, Mesa, Arizona 85212 (United States)
  • 2. School of Chemistry, Tel Aviv University, Tel Aviv IL-69978 (Israel)

Description

We consider the interaction of electromagnetic radiation of arbitrary polarization with multilevel atoms in a self-consistent manner, taking into account both spatial and temporal dependencies of local fields. This is done by numerically solving the corresponding system of coupled Maxwell-Liouville equations for various geometries. In particular, we scrutinize linear optical properties of nanoscale atomic clusters, demonstrating the significant role played by collective effects and dephasing. It is shown that subwavelength atomic clusters exhibit two resonant modes, one of which is localized slightly below the atomic transition frequency of an individual atom, while the other is positioned considerably above it. As an initial exploration of future applications of this approach, the optical response of core-shell nanostructures, with a core consisting of silver and a shell composed of resonant atoms, is examined.

Additional details

Publishing Information

Journal Title
Physical Review. A
Journal Volume
84
Journal Issue
4
Journal Page Range
p. 043802-043802.10
ISSN
1050-2947
CODEN
PLRAAN

Optional Information

Notes
(c) 2011 American Institute of Physics