Published November 1995 | Version v1
Journal article

Orthorhombic to tetragonal transition and appearance of superconductivity in Nd0.7Pr0.3Ba2-kSrkCu3O6+z (0≤k≤1)

  • 1. CNRS, Meudon (France). Lab. de Physique des Solides de Bellevue
  • 2. Univ. de Paris Sud, Orsay (France). Lab. de Chimie des Solides

Description

Preparation, X-ray diffraction and ac susceptibility of Nd0.7Pr0.3Ba2-kSrkCu3O6+z (0 ≤ k ≤ 1) are reported. An orthorhombic to tetragonal transition was observed for k ≥ 0.75. Superconductivity occurred only for k≥0.25. When the samples were heated in argon prior to oxygen annealing both the orthorhombicity (for 0 ≤ k ≤ 0.75) and Tc increased (by 10 K for k = 1). Though a weakening of Pr-f hybridization with Cu-O bands due to Sr substitution may explain the data, a detailed knowledge of oxygen defect chemistry will be required to understand the behavior of Pr in LnBa2Cu3O6+z (Ln = rare earths)

Additional details

Publishing Information

Journal Title
Materials Research Bulletin
Journal Volume
30
Journal Issue
11
Journal Page Range
p. 1363-1370.
ISSN
0025-5408
CODEN
MRBUAC