Variation in airborne ¹³⁴Cs, ¹³⁷Cs, particulate ¹³¹I and ⁷Be maximum activities at high-altitude European locations after the arrival of Fukushima-labeled air masses

The Fukushima-labeled air mass arrival, and later the cesium-134 (¹³⁴Cs), cesium-137 (¹³⁷Cs) and particulate iodine-131 (hereafter noted ¹³¹I_p) maximum levels were registered in Europe at different dates depending on the location. Most of those data were obtained at low-altitude sampling areas. Here, we compare the airborne levels registered at different high-altitude European locations (from 850 m to about 3500 m). The integrated ¹³⁷Cs activity concentration was not uniform with regard to the altitude even after a long travel time/distance from Japan. Moreover, the relation of integrated ¹³⁷Cs vs. altitude showed a linear decrease up to an altitude of about 3000 m. A similar trend was noticed for ¹³¹I_p (particulate fraction) while it increased above 3000 m. Comparison with ⁷Be activity concentration showed that, as far as the high altitude location is concerned, the ¹³⁷Cs and ¹³⁴Cs maximum concentrations corresponded to the ⁷Be maximum, suggesting downdraft movements from high tropospheric or stratospheric layers to be responsible for ^137,134Cs increase and peak values. This was also confirmed by high potential vorticity and low relative humidity registered during the peak values. - Highlights: • Airborne radionuclides from the FDNPP accident, at high-altitude locations across Europe. • Total amount of ¹³⁷Cs that passed was not homogeneous with regard to the altitude. • Peak concentrations were due to downdrafts as revealed by ⁷Be maximum and potential vorticity. • In accident situation, gaseous ¹³¹I monitoring should be more widely performed as for aerosols.