Comparative study of radiation-induced luminescence properties in Eu:SrAl2O4 translucent ceramic and single crystal
Creators
- 1. Division of Materials Science, Nara Institute of Science and Technology (NAIST), 8916-5 Takayama, Ikoma, Nara, 630-0192 (Japan)
- 2. Department of Applied Chemistry, Kanazawa Institute of Technology, 7-1 Ohgigaoka, Nonoichi, Ishikawa, 921 - 8501 (Japan)
Description
Highlights: • A Eu-doped SrAl2O4 translucent ceramic was successfully synthesized by the spark plasma sintering technique. • Comparative studies of the radiation induced luminescence properties were performed. • The synthesized Eu-doped SrAl2O4 translucent ceramic shows the highest transmittance ever. • There is a negative correlation between scintillation and storage luminescence properties. -- Abstract: A Eu-doped SrAl2O4 translucent ceramic was synthesized by the spark plasma sintering technique while a single crystal was grown by the floating zone method. Further, comparative studies of the scintillation and ionizing radiation-induced storage luminescence properties were performed. The transmittance of the synthesized ceramic is 60–70%, which is close to that of the single crystal. Both materials exhibit photoluminescence and scintillation predominantly with a broad emission peaking around 510 nm. The obtained decay time constants confirm that the major origin of the emission is the 5 d-4f transitions of Eu2+, and the decay curve of the ceramic sample indicates the presence of the emission due to some kinds of defects. From the pulse height spectra measured under 137Cs gamma-ray irradiation, the light yields of the single crystal and ceramic are 29,000 and 5700 photons/MeV, respectively. As storage luminescence properties, thermoluminescence and afterglow properties were also evaluated.
Additional details
Identifiers
- DOI
- 10.1016/j.radmeas.2019.106127;
- PII
- S1350448719302422;
Publishing Information
- Journal Title
- Radiation Measurements
- Journal Volume
- 126
- Journal Page Range
- vp.
- ISSN
- 1350-4487
- CODEN
- RMEAEP
INIS
- Country of Publication
- United Kingdom
- Country of Input or Organization
- International Atomic Energy Agency (IAEA)
- INIS RN
- 55075722
- Subject category
- S61: RADIATION PROTECTION AND DOSIMETRY;
- Descriptors DEI
- AFTERGLOW; CERAMICS; CESIUM 137; CORRELATIONS; DECAY; DEFECTS; DOPED MATERIALS; DOSIMETRY; EUROPIUM IONS; GAMMA RADIATION; IRRADIATION; MONOCRYSTALS; PHOTOLUMINESCENCE; PLASMA; SCINTILLATIONS; SINTERING; THERMOLUMINESCENCE
- Descriptors DEC
- BETA DECAY RADIOISOTOPES; BETA-MINUS DECAY RADIOISOTOPES; CESIUM ISOTOPES; CHARGED PARTICLES; CRYSTALS; ELECTROMAGNETIC RADIATION; EMISSION; FABRICATION; INTERMEDIATE MASS NUCLEI; IONIZING RADIATIONS; IONS; ISOTOPES; LUMINESCENCE; MATERIALS; NUCLEI; ODD-EVEN NUCLEI; PHOTON EMISSION; RADIATIONS; RADIOISOTOPES; YEARS LIVING RADIOISOTOPES
Optional Information
- Copyright
- Copyright (c) 2019 Elsevier Ltd. All rights reserved.