Published April 21, 2008
| Version v1
Journal article
Propagation of complex shaped ultrafast pulses in highly optically dense samples
- 1. Department of Chemistry, Princeton University, Princeton, New Jersey 08544 (United States)
- 2. Department of Chemistry, Duke University, Durham, North Carolina 27708 (United States)
- 3. Department of Chemistry, Indian Institute of Technology, Kanpur 208016 (India)
Description
We examine the propagation of shaped (amplitude- and frequency-modulated) ultrafast laser pulses through optically dense rubidium vapor. Pulse reshaping, stimulated emission dynamics, and residual electronic excitation all strongly depend on the laser pulse shape. For example, frequency swept pulses, which produce adiabatic passage in the optically thin limit (independent of the sign of the frequency sweep), behave unexpectedly in optically dense samples. Paraxial Maxwell optical Bloch equations can model our ultrafast pulse propagation results well and provide insight
Additional details
Identifiers
- DOI
- 10.1063/1.2894871;
Publishing Information
- Journal Title
- Journal of Chemical Physics
- Journal Volume
- 128
- Journal Issue
- 15
- Journal Page Range
- p. 154312-154312.14
- ISSN
- 0021-9606
- CODEN
- JCPSA6
INIS
- Country of Publication
- United States
- Country of Input or Organization
- International Atomic Energy Agency (IAEA)
- INIS RN
- 39113855
- Subject category
- S71: CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSICS;
- Descriptors DEI
- BLOCH EQUATIONS; FREQUENCY MODULATION; PULSE SHAPERS; PULSES; RUBIDIUM; STIMULATED EMISSION; VAPORS
- Descriptors DEC
- ALKALI METALS; ELECTRONIC CIRCUITS; ELEMENTS; EMISSION; ENERGY-LEVEL TRANSITIONS; EQUATIONS; FLUIDS; GASES; METALS; MODULATION; PULSE CIRCUITS; SIGNAL CONDITIONERS
Optional Information
- Notes
- (c) 2008 American Institute of Physics