Published April 21, 2008 | Version v1
Journal article

Propagation of complex shaped ultrafast pulses in highly optically dense samples

  • 1. Department of Chemistry, Princeton University, Princeton, New Jersey 08544 (United States)
  • 2. Department of Chemistry, Duke University, Durham, North Carolina 27708 (United States)
  • 3. Department of Chemistry, Indian Institute of Technology, Kanpur 208016 (India)

Description

We examine the propagation of shaped (amplitude- and frequency-modulated) ultrafast laser pulses through optically dense rubidium vapor. Pulse reshaping, stimulated emission dynamics, and residual electronic excitation all strongly depend on the laser pulse shape. For example, frequency swept pulses, which produce adiabatic passage in the optically thin limit (independent of the sign of the frequency sweep), behave unexpectedly in optically dense samples. Paraxial Maxwell optical Bloch equations can model our ultrafast pulse propagation results well and provide insight

Additional details

Identifiers

Publishing Information

Journal Title
Journal of Chemical Physics
Journal Volume
128
Journal Issue
15
Journal Page Range
p. 154312-154312.14
ISSN
0021-9606
CODEN
JCPSA6

INIS

Country of Publication
United States
Country of Input or Organization
International Atomic Energy Agency (IAEA)
INIS RN
39113855
Subject category
S71: CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSICS;
Descriptors DEI
BLOCH EQUATIONS; FREQUENCY MODULATION; PULSE SHAPERS; PULSES; RUBIDIUM; STIMULATED EMISSION; VAPORS
Descriptors DEC
ALKALI METALS; ELECTRONIC CIRCUITS; ELEMENTS; EMISSION; ENERGY-LEVEL TRANSITIONS; EQUATIONS; FLUIDS; GASES; METALS; MODULATION; PULSE CIRCUITS; SIGNAL CONDITIONERS

Optional Information

Notes
(c) 2008 American Institute of Physics