Published January 2014 | Version v1
Journal article

Kinetic model for electrorefining, part II: Model applications and case studies

  • 1. Los Alamos National Laboratory (United States)
  • 2. The Ohio State University, Department of Mechanical and Aerospace Engineering, Nuclear Engineering Program (United States)

Description

The model developed in Part I of the systematic study is applied to identify the kinetic features of materials flow in an electrorefinner. The most recent thermodynamic and electrochemical data reported are used in the present simulations. Both liquid and solid electrodes are considered. The main differences of the kinetics of materials dissolution/deposition between the liquid and solid electrode and the reasons for these differences are identified. The important factors that affect the evolution of electrorefining with operation are identified.

Availability note (English)

Available from http://dx.doi.org/10.1016/j.pnucene.2013.03.008

Additional details

Identifiers

DOI
10.1016/j.pnucene.2013.03.008;
PII
S014919701300053X;

Publishing Information

Journal Title
Progress in Nuclear Energy
Journal Volume
70
Journal Page Range
p. 287-297
ISSN
0149-1970

INIS

Country of Publication
United Kingdom
Country of Input or Organization
International Atomic Energy Agency (IAEA)
INIS RN
51011088
Subject category
S11: NUCLEAR FUEL CYCLE AND FUEL MATERIALS; S38: RADIATION CHEMISTRY, RADIOCHEMISTRY AND NUCLEAR CHEMISTRY;
Descriptors DEI
DEPOSITION; DISSOLUTION; ELECTROCHEMISTRY; ELECTRODES; ELECTROREFINING; FUEL CYCLE; LIQUIDS; REACTION KINETICS; SIMULATION; SOLIDS; THERMODYNAMICS
Descriptors DEC
CHEMISTRY; ELECTROLYSIS; FLUIDS; KINETICS; LYSIS; PROCESSING; REFINING

Optional Information

Notes
Copyright © 2013 Elsevier Ltd. All rights reserved.