Published March 2010 | Version v1
Journal article

Lifetimes and branching ratios of excited states in La-, Os-, Lu-, Lr-, and Pr-

  • 1. Physics Department, Michigan Technological University, Houghton, Michigan 49931 (United States)

Description

Relativistic configuration-interaction calculations have been performed for all possible E1, M1, and E2 transitions between bound anion states of La- and Os-. We pay particular attention to E1 transitions in each case that may be of use in laser cooling of these anions. Although the La- transition energy is approximately one-third of the Os- transition, our results indicate that the Einstein A coefficient is nearly two orders of magnitude larger, which would lead to more efficient laser cooling. We have also explored long-lived opposite-parity excited states in Lu- and Lr- which are restricted to M2 decay by selection rules. Finally, in Pr-, we find sufficient mixing between a weakly bound excited 4f25d26s2 state with a nearby 4f36s26p resonance to result in a lifetime similar to that of the other excited anion states, despite the fact that the dominant configurations of these M1 and E2 transitions differ by two electrons.

Additional details

Identifiers

Publishing Information

Journal Title
Physical Review. A
Journal Volume
81
Journal Issue
3
Journal Page Range
p. 032503-032503.8
ISSN
1050-2947
CODEN
PLRAAN

Optional Information

Notes
(c) 2010 The American Physical Society