Published February 14, 2024 | Version v1
Journal article

Arresting of interfacial phase separation with an imposed flow

  • 1. Department of Chemical Engineering, Tokyo University of Agriculture and Technology, Naka-cho 2-24-16, Koganei, Tokyo 184-8588, Japan
  • 2. PRESTO, Japan Science and Technology Agency, Kawaguchi, Saitama 332-0012, Japan
  • 3. Division of Chemical Engineering, Department of Materials Engineering Science, Graduate School of Engineering Science, Osaka University, Machikaneyamacho 1-3, Toyonaka City, Osaka 560-8531, Japan
  • 4. Department of Mathematics, Indian Institute of Technology Ropar, Rupnagar 140001, India

Description

Using fluid displacement in a Hele-Shaw cell, we experimentally demonstrate the arresting effect of an imposed flow on a phase separation occurring in a growing liquid-liquid interfacial region, unlike in an initially homogeneous single-phase mixture quenched within the miscibility gap. Increasing the imposed flow rate reduces the exponent α in the form ΔAtα, where ΔA is the increase in the area occupied by the displacing fluid owing to phase separation. We show that α can be expressed as a function of the ratio of the phase separation rate to the flow rate on a single curve, indicating that the competition between the imposed flow and phase separation rates determines the degree of the interfacial phase separation. The arresting effect and the mechanism are verified by a numerical simulation.

Additional details

Identifiers

DOI
10.1103/PhysRevFluids.9.024003;
Crossref Funder ID
10.13039/501100001691; 10.13039/501100001695;

Publishing Information

Journal Title
Physical Review Fluids
Journal Volume
9
Journal Issue
2
Journal Page Range
13 pgs.
ISSN
2469-990X

INIS

Country of Publication
United States
Country of Input or Organization
International Atomic Energy Agency (IAEA)
Subject category
S71: CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSICS; S42: ENGINEERING;
Descriptors DEI
AUGMENTATION; COMPUTERIZED SIMULATION; FLOW MODELS; FLOW RATE; FLUID FLOW; FLUID MECHANICS; FLUIDS; INTERFACES; LIQUIDS; MIXTURES; NUMERICAL ANALYSIS; QUENCHING; SOLUBILITY
Descriptors DEC
DISPERSIONS; FLUIDS; MATHEMATICAL MODELS; MATHEMATICS; MECHANICS; SIMULATION

Optional Information

Copyright
©2024 American Physical Society
Contract/Grant/Project number
19K04189; 22K03900; 22K20402; L 19548; JPMJPR22O5
Notes
Contact Email: Corresponding author: ryuta.x.suzuki@gmail.com; Record automatically processed
Funding organization
Japan Society for the Promotion of Science; Japan Science and Technology Corporation