Internal conversion of nuclear transition in the 235mU-C60-nXn molecules and related compounds
Creators
Description
The internal conversion of nuclear transition in the 235U atom is considered. The low-energy γ-quanta (Eγ∼76.8 eV) are emitted during the E3-transition from the excited state (I=(((1)/(2)))+) of the 235U nucleus to its ground state (I=(((7)/(2)))-). The decay rate of this 235mU isomer (E∼76.8 eV) noticeably depends upon the chemical composition and actual physical conditions (i.e. temperature T and pressure p). By varying such a composition and physical conditions one can change the life-time of the 235mU isomer to relatively large/small values. A specific attention is given to the fullerene molecules containing the central 235U atom. It is shown that the decay rate λ of the 235mU isomer in the 235mU-C60-nXn molecules and related compounds can differ significantly from the values obtained for isolated 235U atoms. Some applications of this effect are considered
Additional details
Identifiers
- DOI
- 10.1016/j.radphyschem.2004.05.047;
- PII
- S0969806X04003755;
Publishing Information
- Journal Title
- Radiation Physics and Chemistry (1993)
- Journal Volume
- 72
- Journal Issue
- 5
- Journal Page Range
- p. 541-547
- ISSN
- 0969-806X
- CODEN
- RPCHDM
INIS
- Country of Publication
- United Kingdom
- Country of Input or Organization
- International Atomic Energy Agency (IAEA)
- INIS RN
- 36022149
- Subject category
- S38: RADIATION CHEMISTRY, RADIOCHEMISTRY AND NUCLEAR CHEMISTRY;
- Descriptors DEI
- CHEMICAL COMPOSITION; E3-TRANSITIONS; EV RANGE 10-100; EXCITED STATES; FISSION; FULLERENES; GROUND STATES; INTERNAL CONVERSION; ISOMERIC TRANSITIONS; URANIUM 235
- Descriptors DEC
- ACTINIDE NUCLEI; ALPHA DECAY RADIOISOTOPES; CARBON; CONVERSION; DECAY; ELEMENTS; ENERGY LEVELS; ENERGY RANGE; ENERGY-LEVEL TRANSITIONS; EV RANGE; EVEN-ODD NUCLEI; HEAVY NUCLEI; INTERNAL CONVERSION RADIOISOTOPES; ISOMERIC TRANSITION ISOTOPES; ISOTOPES; MINUTES LIVING RADIOISOTOPES; MULTIPOLE TRANSITIONS; NONMETALS; NUCLEAR DECAY; NUCLEAR REACTIONS; NUCLEI; RADIOISOTOPES; SPONTANEOUS FISSION RADIOISOTOPES; URANIUM ISOTOPES; YEARS LIVING RADIOISOTOPES
Optional Information
- Copyright
- Copyright (c) 2004 Elsevier Science B.V., Amsterdam, The Netherlands, All rights reserved.