Published April 1, 1976 | Version v1
Journal article

Chemical pumping of the water vapor laser. I

  • 1. Department of Chemistry, The Johns Hopkins University, Baltimore, Maryland 21218

Description

Flash photolysis of mixtures of O2/H2O/O3 leads to lasing at 357.53 cm-1. Emission at this wavenumber coincides with that of the strongest line that is observed from both the pulsed and cw water vapor discharge laser. Accordingly it is assigned to the (001)633-- (020)550 transition in water. The pumping scheme O3→/subh//sup nu/O(1D)+O2(1Δ/subg/), (1); O(1D)+O2(3Σ-/subg/) →O2(1Σ+/subg/)+O(3P), (2); O2(1Σ+/subg/)+H2O→O2(1Δ/subg/)+H2O/sup dagger/, (3), where H2O/sup dagger/ subsequently lases, is consistent with all the experimental observations. Computer modeling of this sequence of reactions reproduces both the observed pulse's profile and its onset delay after flash initiation

Additional details

Identifiers

Publishing Information

Journal Title
The Journal of Chemical Physics
Journal Volume
64
Journal Issue
7
Series
J. Chem. Phys.
Journal Page Range
2854-2857
ISSN
0021-9606

INIS

Country of Publication
United States
Country of Input or Organization
United States
INIS RN
7260677
Subject category
S42: ENGINEERING;
Descriptors DEI
CHEMICAL LASERS; ENERGY TRANSFER; GAS LASERS; INFRARED RADIATION; OPERATION; OPTICAL PUMPING; PHOTOLYSIS; WATER VAPOR
Descriptors DEC
AMPLIFIERS; CHEMICAL REACTIONS; DECOMPOSITION; ELECTROMAGNETIC RADIATION; FLUIDS; GASES; LASERS; RADIATIONS; VAPORS

Optional Information

Notes
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