Neutron-induced fission cross sections of short-lived actinides with the surrogate reaction method
Creators
- Jurado, B.1
- Kessedjian, G.1
- Petit, M.1
- Aiche, M.1
- Barreau, G.1
- Bidaud, A.1
- Boyer, S.1
- Carjan, N.1
- Czajkowski, S.1
- Dassie, D.1
- Grosjean, C.1
- Guiral, A.1
- Haas, B.1
- Karamanis, D.1
- Mathieu, L.1
- Misicu, S.1
- Rizea, C.1
- Santiamon, F.1
- Audouin, L.2
- Capellan, N.2
- Tassan-Got, L.2
- Wilson, J.N.2
- Andriamonje, S.3
- Berthoumieux, E.3
- Bouchez, E.3
- Gunsing, F.3
- Hurstel, A.3
- Lecoz, Y.3
- Lucas, R.3
- Theisen, C.3
- Serot, O.4
- Bauge, E.5
- Billebaud, A.6
- Perrot, L.6
- Ahmad, I.7
- Greene, J.P.7
- Jansens, R.V.F.7
- 1. CENBG, Chemin du Solarium B.P. 120, 33175 Gradignan (France)
- 2. IPN, Universite de Paris-Sud, 91405 Orsay (France)
- 3. CEA-Saclay, DSM/DAPNIA/SPhN, 91191 Gif-sur-Yvette cedex (France)
- 4. CEA-Cadarache, DEN/DER/SPRC/LEPh, 13108 Saint Paul lez Durance (France)
- 5. CEA DAM DIF, 91297 Arpajon (France)
- 6. LPSC, 38026 Grenoble cedex (France)
- 7. Physics Division, Argonne National Laboratory, 9700 S. Cass Avenue, IL 60439 (United States)
Description
We present a review of the fission cross section measurements made by the CENBG collaboration over the last years using the surrogate reaction method. For example the neutron-induced fission cross sections of 233Pa (T1/2=27 d), 242Cm (T1/2=162.8 d) and 243Cm (T1/2=29.1 y) have been obtained by our group with this technique. The advantages and the difficulties of the surrogate method are discussed. Special attention is paid to the comparison between cross sections measured with the surrogate method and those obtained directly with neutrons at low energies. This comparison provides information on possible differences between the spin-parity distributions achieved in the two methods. We measured for the first time the fission cross section of 233Pa. Our results for 231Pa(n,f) revealed that the existing neutron-induced data overestimated the fission cross section above 1.5 MeV. The deduced 241Am(n,f) and 242Cm(n,f) cross sections agree with the available data obtained via neutron-induced reactions. The good agreement observed at the lowest neutron energies between the present results and the neutron-induced data for 242Cm(n,f) and 243Cm(n,f) indicates that the population of excited states generated by the transfer reactions used in this work is similar to the distribution fed in neutron induced reactions. This agreement illustrates the potential of the surrogate reaction method to provide neutron-induced fission cross sections for short-lived nuclei
Availability note (English)
Available from doi: http://dx.doi.org/10.1051/epjconf/20100206004Additional details
Identifiers
Publishing Information
- Publisher
- EDP Sciences
- Imprint Place
- Les Ulis (France)
- ISBN
- 978-2-7598-0521-1
- Imprint Title
- EPJ Web of Conferences, Proceedings of the Second International Workshop on Compound Nuclear Reactions and Related Topics - CNR*09. V. 2
- Imprint Pagination
- 290 p.
- Journal Page Range
- p. 06004-1.06004
Conference
- Title
- 2. International Workshop on Compound Nuclear Reactions and Related Topics
- Acronym
- CNR 09
- Dates
- 5-8 Oct 2009
- Place
- Bordeaux (France)
INIS
- Country of Publication
- France
- Country of Input or Organization
- France
- INIS RN
- 44029392
- Subject category
- S73: NUCLEAR PHYSICS AND RADIATION PHYSICS;
- Resource subtype / Literary indicator
- Conference
- Descriptors DEI
- ACTINIDES; AMERICIUM 241; CROSS SECTIONS; CURIUM 242; CURIUM 243; EXCITED STATES; FISSION; MEV RANGE; NEUTRON REACTIONS; PROTACTINIUM 231; PROTACTINIUM 233; SPIN; TRANSFER REACTIONS
- Descriptors DEC
- ACTINIDE NUCLEI; ALPHA DECAY RADIOISOTOPES; AMERICIUM ISOTOPES; ANGULAR MOMENTUM; BARYON REACTIONS; BETA DECAY RADIOISOTOPES; BETA-MINUS DECAY RADIOISOTOPES; CURIUM ISOTOPES; DAYS LIVING RADIOISOTOPES; DIRECT REACTIONS; ELEMENTS; ENERGY LEVELS; ENERGY RANGE; EVEN-EVEN NUCLEI; EVEN-ODD NUCLEI; HADRON REACTIONS; HEAVY ION DECAY RADIOISOTOPES; HEAVY NUCLEI; ISOTOPES; METALS; NEON 24 DECAY RADIOISOTOPES; NUCLEAR REACTIONS; NUCLEI; NUCLEON REACTIONS; ODD-EVEN NUCLEI; PARTICLE PROPERTIES; PROTACTINIUM ISOTOPES; RADIOISOTOPES; SPONTANEOUS FISSION RADIOISOTOPES; YEARS LIVING RADIOISOTOPES
Optional Information
- Notes
- 23 refs.