Time-dependent theory of reconstruction of attosecond harmonic beating by interference of multiphoton transitions
- 1. Instituto de Investigaciones en Energía No Convencional - INENCO (UNSa - CONICET), Av. Bolivia 5150, 4400, Salta Capital, Argentina
- 2. Institute for Astronomy and Space Physics - IAFE (UBA-CONICET), C1428GA, Buenos Aires, Argentina
- 3. Universidad de Buenos Aires, Facultad de Ciencias Exactas y Naturales y Ciclo Básico Común, C1428EGA Buenos Aires, Argentina
Description
Phase and time delays of atomic above-threshold ionization are usually experimentally explored by the reconstruction of attosecond harmonic beating by interference of two-photon transitions (RABBIT) technique. Theoretical studies of RABBIT rely on the perturbative treatment of the probe (near infrared or visible) laser pulse with respect to the atomic electric field and the pump composed of a train of attosecond pulses made of several harmonics with frequencies multiple of the probe fundamental frequency. In this work we present a semiclassical nonperturbative description of the phase delays for the emission of electrons from hydrogen atoms based on the strong-field approximation as the relative phase between pump and probe pulses is varied, where more than two photons are involved. Ionization times are calculated within the saddle-point approximations and serve to individualize the different electron wave packets that produce the RABBIT-like interferometric scheme. We observe different behaviors of the phase delays at different intensities of the probe. For example, for moderate and intense probe fields, the harmonics and sidebands happen to be in phase (). In turn, when the probe field is sufficiently weak, we recover the well-known rule of thumb for the phase delays developed within the perturbative RABBIT theory [see D. Guénot et al., Phys. Rev. A 85, 053424 (2012)]. We show that the intracycle interference of the different paths contributing to the final energy (sideband or high harmonic) is responsible for the different behaviors of the interference pattern. Comparisons with the numerical solution of the strong-field approximation and time-dependent Schrödinger equation confirm the reliability of our semiclassical nonperturbative theory.
Additional details
Identifiers
- DOI
- 10.1103/PhysRevA.110.013104;
- arXiv
- arXiv:2401.04299;
- Crossref Funder ID
- 10.13039/501100003074; 10.13039/501100002923; 10.13039/501100003033;
Publishing Information
- Journal Title
- Physical Review A
- Journal Volume
- 110
- Journal Issue
- 1
- Journal Page Range
- 15 pgs.
- ISSN
- 1094-1622
INIS
- Country of Publication
- United States
- Country of Input or Organization
- International Atomic Energy Agency (IAEA)
- Subject category
- S74: ATOMIC AND MOLECULAR PHYSICS; S71: CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSICS;
- Descriptors DEI
- APPROXIMATIONS; ELECTRIC FIELDS; HARMONICS; HYDROGEN; INTERFERENCE; INTERFEROMETERS; INTERFEROMETRY; NUMERICAL SOLUTION; OPTICAL PUMPING; PHOTOIONIZATION; PROBES; PULSES; SCHROEDINGER EQUATION; SEMICLASSICAL APPROXIMATION; TIME DEPENDENCE; WAVE PACKETS
Optional Information
- Copyright
- ©2024 American Physical Society
- Contract/Grant/Project number
- 2020-01755; 2020-01434; 2022-2024 11220210100468CO
- Notes
- Contact Email: Contact author: sebastian.lopez@conicet.gov.ar; Record automatically processed
- Funding organization
- Agencia Nacional de Promoción Científica y Tecnológica; Consejo Nacional de Investigaciones Científicas y Técnicas; Ministerio de Ciencia, Tecnología e Innovación