Burnup dependence of melting temperature of FBR mixed oxide fuels irradiated to high burnup
Creators
- 1. Oarai Research and Development Center, Japan Atomic Energy Agency, 4002 Narita-cho, Oarai-machi, Higashiibaraki-gun, Ibaraki 311-1393 (Japan)
Description
Highlights: → Melting temperatures for irradiated MOX fuels were measured by a new method. → In the new method, a rhenium inner capsule is used to stop fuel-tungsten reactions. → Melting temperatures of irradiated MOX fuels linearly-decrease depending on burnup. → The decrease mainly results from solid solution of fission products in fuels. - Abstract: The melting temperatures of FBR MOX fuels with Pu content of 28-30 wt.% irradiated to from 22.5 to 112.5 MWd kg-1 were measured using a rhenium inner capsule to hold the specimens. The rhenium inner capsule could prevent chemical reactions between fuels and tungsten materials which decrease the melting temperature. The melting temperatures were about 30 K higher than the previous data using tungsten capsules. The melting temperature decreases in a linear manner with burnup due to solid solution of fission products in fuels. However, the slopes of the lines plotting melting temperature versus burnup are almost similar to the previous data.
Availability note (English)
Available from http://dx.doi.org/10.1016/j.jnucmat.2011.07.001Additional details
Identifiers
- DOI
- 10.1016/j.jnucmat.2011.07.001;
- PII
- S0022-3115(11)00650-7;
Publishing Information
- Journal Title
- Journal of Nuclear Materials
- Journal Volume
- 418
- Journal Issue
- 1-3
- Journal Page Range
- p. 207-214
- ISSN
- 0022-3115
- CODEN
- JNUMAM
INIS
- Country of Publication
- Netherlands
- Country of Input or Organization
- International Atomic Energy Agency (IAEA)
- INIS RN
- 43060018
- Subject category
- S11: NUCLEAR FUEL CYCLE AND FUEL MATERIALS; S36: MATERIALS SCIENCE;
- Descriptors DEI
- BURNUP; CAPSULES; CHEMICAL REACTIONS; FISSION PRODUCTS; MELTING POINTS; MIXED OXIDE FUELS; RHENIUM; SOLID SOLUTIONS; TUNGSTEN
- Descriptors DEC
- CONTAINERS; DISPERSIONS; ELEMENTS; ENERGY SOURCES; FUELS; HOMOGENEOUS MIXTURES; ISOTOPES; MATERIALS; METALS; MIXTURES; NUCLEAR FUELS; PHYSICAL PROPERTIES; RADIOACTIVE MATERIALS; REACTOR MATERIALS; REFRACTORY METALS; SOLID FUELS; SOLUTIONS; THERMODYNAMIC PROPERTIES; TRANSITION ELEMENTS; TRANSITION TEMPERATURE
Optional Information
- Copyright
- Copyright (c) 2011 Elsevier Science B.V., Amsterdam, The Netherlands, All rights reserved.