Light-Induced Melting of Competing Stripe Orders without Introducing Superconductivity in
Creators
- 1. International Center for Quantum Materials, School of Physics, Peking University, Beijing 100871, China
- 2. National Synchrotron Light Source II, Brookhaven National Laboratory, Upton, New York 11973, USA
Description
The ultrafast manipulation of quantum material has led to many novel and significant discoveries. Among them, the light-induced transient superconductivity in cuprates achieved by melting competing stripe orders represents a highly appealing accomplishment. However, recent investigations have shown that the notion of photoinduced superconductivity remains a topic of controversy, and its elucidation solely through -axis time-resolved terahertz spectroscopy remains an arduous task. Here, we measure the in-plane and out-of-plane transient terahertz responses simultaneously in the stripe-ordered nonsuperconducting after near-infrared excitations. We find that although a pump-induced reflectivity edge appears in the -axis reflectance spectrum, the reflectivity along the planes decreases simultaneously, indicating an enhancement in the scattering rate of quasiparticles. This in-plane transient response is clearly distinct from the features associated with superconducting condensation. Therefore, we conclude the out-of-plane transient responses cannot be explained by an equivalent of Josephson tunneling. Notably, those pump-induced terahertz responses remain consistent even when we vary the near-infrared optical pump wavelengths and hole concentrations. Our results provide critical evidence that transient three-dimensional superconductivity cannot be induced by melting the competing stripe orders with pump pulses whose photon energy is much higher than the superconducting gap of cuprates.
Files
10.1103_PhysRevX.14.011036.pdf
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(11.7 MB)
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Additional details
Identifiers
- DOI
- 10.1103/PhysRevX.14.011036;
- arXiv
- arXiv:2306.07869;
- Crossref Funder ID
- 10.13039/501100001809; 10.13039/501100012166; 10.13039/100006231; 10.13039/100006132; 10.13039/100000015;
Publishing Information
- Journal Title
- Physical Review X
- Journal Volume
- 14
- Journal Issue
- 1
- Journal Page Range
- 11 pgs.
- ISSN
- 2160-3308
INIS
- Country of Publication
- United States
- Country of Input or Organization
- International Atomic Energy Agency (IAEA)
- Subject category
- S75: CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND SUPERFLUIDITY;
- Descriptors DEI
- BARIUM OXIDES; COPPER OXIDES; CUPRATES; EXCITATION; HOLES; JOSEPHSON JUNCTIONS; LANTHANUM COMPOUNDS; LANTHANUM OXIDES; MELTING; PULSES; REFLECTIVITY; SPECTROSCOPY; SUPERCONDUCTIVITY; TRANSIENTS; TUNNEL EFFECT; WAVELENGTHS
- Descriptors DEC
- BARIUM COMPOUNDS; CHALCOGENIDES; COPPER COMPOUNDS; ELECTRIC CONDUCTIVITY; ELECTRICAL PROPERTIES; ENERGY-LEVEL TRANSITIONS; LANTHANUM COMPOUNDS; OPTICAL PROPERTIES; OXIDES; OXYGEN COMPOUNDS; PHASE TRANSFORMATIONS; PHYSICAL PROPERTIES; RARE EARTH COMPOUNDS; SUPERCONDUCTING JUNCTIONS; SURFACE PROPERTIES; TRANSITION ELEMENT COMPOUNDS; TUNNEL JUNCTIONS
Optional Information
- Contract/Grant/Project number
- 11888101; 12304184; 2022YFA1403901; DE-SC0012704
- Notes
- Contact Email: sjzh@pku.edu.cn; Contact Email: nlwang@pku.edu.cn; Record automatically processed
- Funding organization
- National Natural Science Foundation of China; National Key Research and Development Program of China; Brookhaven National Laboratory; Office of Science; U.S. Department of Energy