Published March 4, 2024 | Version v1
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Light-Induced Melting of Competing Stripe Orders without Introducing Superconductivity in La2xBaxCuO4

  • 1. International Center for Quantum Materials, School of Physics, Peking University, Beijing 100871, China
  • 2. National Synchrotron Light Source II, Brookhaven National Laboratory, Upton, New York 11973, USA

Description

The ultrafast manipulation of quantum material has led to many novel and significant discoveries. Among them, the light-induced transient superconductivity in cuprates achieved by melting competing stripe orders represents a highly appealing accomplishment. However, recent investigations have shown that the notion of photoinduced superconductivity remains a topic of controversy, and its elucidation solely through c-axis time-resolved terahertz spectroscopy remains an arduous task. Here, we measure the in-plane and out-of-plane transient terahertz responses simultaneously in the stripe-ordered nonsuperconducting La2xBaxCuO4 after near-infrared excitations. We find that although a pump-induced reflectivity edge appears in the c-axis reflectance spectrum, the reflectivity along the CuO2 planes decreases simultaneously, indicating an enhancement in the scattering rate of quasiparticles. This in-plane transient response is clearly distinct from the features associated with superconducting condensation. Therefore, we conclude the out-of-plane transient responses cannot be explained by an equivalent of Josephson tunneling. Notably, those pump-induced terahertz responses remain consistent even when we vary the near-infrared optical pump wavelengths and hole concentrations. Our results provide critical evidence that transient three-dimensional superconductivity cannot be induced by melting the competing stripe orders with pump pulses whose photon energy is much higher than the superconducting gap of cuprates.

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10.1103_PhysRevX.14.011036.pdf

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Additional details

Identifiers

DOI
10.1103/PhysRevX.14.011036;
arXiv
arXiv:2306.07869;
Crossref Funder ID
10.13039/501100001809; 10.13039/501100012166; 10.13039/100006231; 10.13039/100006132; 10.13039/100000015;

Publishing Information

Journal Title
Physical Review X
Journal Volume
14
Journal Issue
1
Journal Page Range
11 pgs.
ISSN
2160-3308

Optional Information

Contract/Grant/Project number
11888101; 12304184; 2022YFA1403901; DE-SC0012704
Notes
Contact Email: sjzh@pku.edu.cn; Contact Email: nlwang@pku.edu.cn; Record automatically processed
Funding organization
National Natural Science Foundation of China; National Key Research and Development Program of China; Brookhaven National Laboratory; Office of Science; U.S. Department of Energy