Published 1991 | Version v1
Miscellaneous

Models for multiphoton ionization processes

Description

Using the Fourier transform method, several analytical models for multiphoton processes have been developed, which emphasize the non-perturbative regime of C-C transitions. It was found that the population trapping of continuum-continuum (C-C) transitions can occurs under general conditions: for two continua with energy-dependent matrix elements, and for an infinite number of structureless continua with coupled bands. A above-threshold ionization model with two-frequency smooth pulses for hydrogenic atom was first proposed. This model give a simple form for analytical solutions if an ionization threshold is negligible. The results predict that (a) there is no trapping or saturation of the bound-continuum transition and that the ionization rate is independent of the redistribution among the continua for the C-C matrix element chosen; (b) There are peak switch in photoelectron energy spectra which depends on not only redistribution laser intensity, but also the pulses shape and their overlap in time, as well as the coupling between the bound state and continua; (c) peaks about the ionization energy in the photoelectron spectra are symmetric and only appear during the ionization process; (d) as the laser intensity is increased, the total angular photoelectrons distribution peak strongly in forward and backward direction of the redistribution laser polarization; and the minima of this distribution are not zero for higher laser intensity. The photon spectrum is also investigated

Availability note (English)

University Microfilms, PO Box 1764, Ann Arbor, MI 48106, Order No.92-02,217.

Additional details

Publishing Information

Publisher
Rensselaer Polytechnic Inst.
Imprint Place
Troy. NY (United States)
Imprint Pagination
134 p.

INIS

Country of Publication
United States
Country of Input or Organization
United States
INIS RN
23069204
Subject category
S74: ATOMIC AND MOLECULAR PHYSICS;
Resource subtype / Literary indicator
Thesis, Non-conventional Literature
Descriptors DEI
ANALYTICAL SOLUTION; ENERGY SPECTRA; IONIZATION; LASER RADIATION; MATHEMATICAL MODELS; MATRIX ELEMENTS; MULTI-PHOTON PROCESSES; PERTURBATION THEORY; PHOTOELECTRON SPECTROSCOPY
Descriptors DEC
ELECTROMAGNETIC RADIATION; ELECTRON SPECTROSCOPY; RADIATIONS; SPECTRA; SPECTROSCOPY