Published July 1992 | Version v1
Journal article

Calculation of thermodynamic properties of liquid and amorphous oxides 2MeOxSiO2 (Me = Mg, Fe, Ca, Sr, Ba)

  • 1. Moskovskij Inst. Stali i Splavov, Moscow (Russian Federation)

Description

Methods of continuous static relaxation and molecular dynamics were used to calculate changes of volume, energy, Gibbs energy, and entropy under formation of oxides of 2MeOxSiO2 series from simple MeO (Me = Mg, Fe, Ca, Sr, Ba) and SiO2 oxides at 0 and 2000 K. Only Coulomb interaction and Born-Mayer ion shell repulsion were taken into account. It is shown that rearrangement of oxide structure takes place in the range of ion shell repulsion parameter B13 = 1900-3300 eV; changes of volume and entropy depend on B13 nonmonotonously at that

Additional details

Additional titles

Original title (Russian)
Расчет термодинамических свойств жидких и аморфных оксидов 2MeOxSiO

Publishing Information

Journal Title
Zhurnal Fizicheskoj Khimii
Journal Volume
66
Journal Issue
7
Journal Page Range
p. 1753-1763.
ISSN
0044-4537
CODEN
ZFKHA9