Published May 6, 2024 | Version v1
Journal article

Confinement and magnetic-field effect on chiral ferroelectric nematic liquid crystals in Grandjean-Cano wedge cells

  • 1. Advanced Materials and Liquid Crystal Institute, Kent State University, Kent, Ohio 44242, USA
  • 2. Department of Physics, Kent State University, Kent, Ohio 44242, USA
  • 3. Materials Science Graduate Program, Kent State University, Kent, Ohio 44242, USA

Description

We explore the structure and magnetic-field response of edge dislocations in Grandjean-Cano wedge cells filled with chiral mixtures of the ferroelectric nematic mesogen DIO. Upon cooling, the ordering changes from paraelectric in the cholesteric phase N* to antiferroelectric in the smectic SmZA* and to ferroelectric in the cholesteric NF*. Dislocations of the Burgers vector b equal to the helicoidal pitch P are stable in all three phases, while dislocations with b=P/2 exist only in the N* and SmZA*. The b=P/2 dislocations split into pairs of τ1/2λ+1/2 disclinations, while the thick dislocations b=P are pairs of nonsingular λ1/2λ+1/2 disclinations. The polar order makes the τ1/2 disclinations unstable in the NF* phase, as they should be connected to singular walls in the polarization field. We propose a model of transformation of the composite τ1/2 line-wall defect into a nonsingular λ1/2 disclination, which is paired up with a λ+1/2 line to form a b=P dislocation. The SmZA* behavior in the in-plane magnetic field is different from that of the NF* and N*: the dislocations show no zigzag instability, and the pitch remains unchanged in the magnetic fields up to 1 T. The behavior is associated with the finite compressibility of smectic layers.

Additional details

Identifiers

DOI
10.1103/PhysRevE.109.054702;
arXiv
arXiv:2403.20229;
Crossref Funder ID
10.13039/100000001;

Publishing Information

Journal Title
Physical Review E
Journal Volume
109
Journal Issue
5
Journal Page Range
14 pgs.
ISSN
1089-3787

Optional Information

Copyright
©2024 American Physical Society
Contract/Grant/Project number
ECCS-2122399; DMR-2210083
Notes
Contact Email: olavrent@kent.edu; Record automatically processed
Funding organization
National Science Foundation