Published March 2015 | Version v1
Journal article

Synthesis and crystal and molecular structure of three heterometallic polymeric compounds (Ln2[LnGe6(μ-Oedph)6(μ-O)3(μ-OH)3(H2O)4] · xH2O)n [Ln = Nd, x ∼ 26 (I); Er, x ∼ 24 (II); Tm, x ∼ 20 (III); H4Oedph = 1-hydroxyethylidenediphosphonic acid]

  • 1. Russian Academy of Sciences, Kurnakov Institute of General and Inorganic Chemistry (Russian Federation)
  • 2. Mechnikov Odessa National University (Ukraine)

Description

The synthesis and X-ray diffraction study of three heterometallic compounds of general formula (Ln2[LnGe6(μ-Oedph)6(μ-O)3(μ-OH)3(H2O)4] · xH2O)n [Ln = Nd, x ∼ 26 (I); Er, x ∼ 24 (II); Tm, x ∼20 (III); H4Oedph = 1-hydroxyethylidenediphosphonic acid] are performed. The basis element of structures I–III is a hexanuclear complex anion [Ge(μ-Oedph)(μ-O)0.5(μ-OH)0.5]69−, in which bridging hydroxo and oxo ligands are statistically disordered with equally probability. Hexameric units are connected by Ln1(H2O)4 fragments into a framework whose channels are completely populated by disordered lanthanide atoms and water molecules

Additional details

Identifiers

Publishing Information

Journal Title
Crystallography Reports
Journal Volume
60
Journal Issue
2
Journal Page Range
p. 204-209
ISSN
1063-7745
CODEN
CYSTE3

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