Revisiting the heavy-fermion compound : Kondo temperature and the ground-state degeneracy
Creators
- 1. Department of Physics, Simon Fraser University, Burnaby, British Columbia, Canada V5A 1S6
Description
has been characterized as a heavy-fermion Kondo lattice system without long-range magnetic order. Thermodynamic and transport data of this compound have been partially analyzed, and the reported Kondo temperatures are highly dependent on samples and estimation methods. In particular, the magnetic susceptibility of this compound does not show the maximum corresponding to the Kondo resonance with a large degeneracy of the ground state, partly due to the sample quality. Thus, single crystals of are grown to reinvestigate their physical properties by means of magnetization, specific heat, electrical resistivity, Hall resistivity, and thermoelectric power measurements. Unlike earlier studies, we found consistencies regarding the K measurement estimated from thermodynamic and transport property measurements. The magnetic part of the specific heat displays a broad maximum near 70 K, which follows well with the prediction made by the Coqblin-Schrieffer (C-S) model for whole multiplets involved in the formation of the Kondo state. However, the local maximum in does not match well with the C-S model prediction due to the crystalline electric field (CEF) effect, where the value is still greater than the overall CEF splittings: . Electrical resistivity and Hall coefficient measurements indicate an extremum near K, while a negative minimum at K is observed in thermoelectric power.
Additional details
Identifiers
- DOI
- 10.1103/PhysRevMaterials.8.013401;
- Crossref Funder ID
- 10.13039/501100001804; 10.13039/501100000038; 10.13039/501100000196;
Publishing Information
- Journal Title
- Physical Review Materials
- Journal Volume
- 8
- Journal Issue
- 1
- Journal Page Range
- 7 pgs.
- ISSN
- 2475-9953
INIS
- Country of Publication
- United States
- Country of Input or Organization
- International Atomic Energy Agency (IAEA)
- Subject category
- S75: CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND SUPERFLUIDITY;
- Descriptors DEI
- ELECTRIC CONDUCTIVITY; ELECTRIC FIELDS; ELECTRONIC SPECIFIC HEAT; FERMIONS; GROUND STATES; HALL EFFECT; KONDO EFFECT; MAGNETIC SPECIFIC HEAT; MAGNETIC SUSCEPTIBILITY; MAGNETIZATION; MONOCRYSTALS; MULTIPLETS; SPECIFIC HEAT; THERMOELECTRICITY; YTTERBIUM ALLOYS
- Descriptors DEC
- ALLOYS; CRYSTALS; ELECTRICAL PROPERTIES; ELECTRICITY; ENERGY LEVELS; MAGNETIC PROPERTIES; PHYSICAL PROPERTIES; RARE EARTH ALLOYS; SPECIFIC HEAT; THERMODYNAMIC PROPERTIES
Optional Information
- Copyright
- ©2024 American Physical Society
- Notes
- Record automatically processed
- Funding organization
- Canada Research Chairs; Natural Sciences and Engineering Research Council of Canada; Canada Foundation for Innovation