Published 2010 | Version v1
Book

Neutron-induced capture cross sections of short-lived actinides with the surrogate reaction method

  • 1. CENBG, Chemin du Solarium, B.P. 120, 33175 Gradignan (France)
  • 2. CEA DAM DIF, F-91297 Arpajon (France)
  • 3. CEA-Cadarache, DEN/DER/SPRC/LEPh, 13108 Saint Paul lez Durance (France)
  • 4. CEA Saclay, DSM/DAPNIA/SPhN, 91191 Gif-sur-Yvette (France)

Description

The determination of neutron-capture cross sections of short-lived nuclei is opening the way to understand and clarify the properties of many nuclei of interest for nuclear structure physics, nuclear astrophysics and particularly for transmutation of nuclear wastes. The surrogate approach is well-recognized as a potentially very useful method to extract neutron cross sections for low-energy compound-nuclear reactions and to overcome the difficulties related to the target radioactivity. In this work we will assess where we stand on these neutron-capture cross section measurements and how we can achieve the short-lived Minor Actinides nuclei involved in the nuclear fuel cycle. The CENBG collaboration applied the surrogate method to determine the neutron-capture cross section of 233Pa (T1/2=27 d). The 233Pa(n,γ) cross section is then deduced from the measured gamma decay probability of 234Pa compound nucleus formed via the surrogate 232Th(3He,p) reaction channel. The obtained cross section data, covering the neutron energy range 0.1 to 1 MeV, have been compared with the predictions of the Hauser-Feshbach statistical model. The importance of establishing benchmarks is stressed for the minor actinides region. However, the lack of desired targets led us to propose recently the 174Yb (3He,pγ) reaction as a surrogate reaction for the (n,γ) predetermined benchmark cross section of 175Lu. An overview of the experimental setup combining gamma ray detectors such as Ge and C6D6 in coincidence with light charged particles ΔE-E Telescopes will be presented and preliminary results will be discussed. (authors)

Availability note (English)

Available from doi: http://dx.doi.org/10.1051/epjconf/20100206002
Part of:
EPJ Web of Conferences, Proceedings of the Second International Workshop on Compound Nuclear Reactions and Related Topics - CNR*09. V. 2

Additional details

Identifiers

Publishing Information

Publisher
EDP Sciences
Imprint Place
Les Ulis (France)
ISBN
978-2-7598-0521-1
Imprint Title
EPJ Web of Conferences, Proceedings of the Second International Workshop on Compound Nuclear Reactions and Related Topics - CNR*09. V. 2
Imprint Pagination
290 p.
Journal Page Range
p. 06002-1.06002

Conference

Title
2. International Workshop on Compound Nuclear Reactions and Related Topics
Acronym
CNR 09
Dates
5-8 Oct 2009
Place
Bordeaux (France)

Optional Information

Notes
9 refs.