Published January 4, 2024 | Version v1
Journal article

Consistency between reflection momentum-resolved electron energy loss spectroscopy and optical spectroscopy measurements of the long-wavelength density response of Bi2Sr2CaCu2O8+x

  • 1. Department of Physics and Materials Research Laboratory, University of Illinois at Urbana-Champaign, Urbana, Illinois 61801, USA
  • 2. Condensed Matter Physics and Materials Science Department, Brookhaven National Laboratory, Upton, New York 11973, USA

Description

The density fluctuation spectrum captures many fundamental properties of strange metals. Using momentum-resolved electron energy loss spectroscopy (M-EELS), we recently showed that the density response of the strange metal Bi2Sr2CaCu2O8+x (Bi-2212) at large momentum, q, exhibits a constant-in-frequency continuum [M. Mitrano et al., Proc. Natl. Acad. Sci. USA 115, 5392 (2018); A. A. Husain et al., Phys. Rev. X 9, 041062 (2019)] reminiscent of the marginal Fermi liquid (MFL) hypothesis of the late 1980s [C. M. Varma et al., Phys. Rev. Lett. 63, 1996 (1989)]. However, reconciling this observation with infrared (IR) optics experiments, which show a well-defined plasmon excitation at q0, has been challenging. Here we report M-EELS measurements of Bi-2212 using 4× improved momentum resolution, allowing us to reach the optical limit. For momenta q<0.04 reciprocal lattice unites (r.l.u.), the M-EELS data show a plasmon feature that is quantitatively consistent with IR optics. For q>0.04 r.l.u., the spectra become incoherent with an MFL-like, constant-in-frequency form. We speculate that, at finite frequency, ω, and nonzero q, some attribute of this Planckian metal randomizes the probe electron, causing it to lose information about its own momentum.

Additional details

Identifiers

DOI
10.1103/PhysRevB.109.045108;
arXiv
arXiv:2306.03681;
Crossref Funder ID
10.13039/100000015; 10.13039/100000001;

Publishing Information

Journal Title
Physical Review B
Journal Volume
109
Journal Issue
4
Journal Page Range
9 pgs.
ISSN
1550-235X

Optional Information

Copyright
©2024 American Physical Society
Contract/Grant/Project number
DE-SC0021238; DE-SC0012704; DMR-2024864
Notes
Contact Email: jinc3@illinois.edu; Contact Email: abbamonte@mrl.illinois.edu; Record automatically processed
Funding organization
U.S. Department of Energy; National Science Foundation