Time gated high order harmonic generation
Description
High Order Harmonic Generation (HHG) is a coherent XUV source obtained by focusing an intense laser pulse into a gas medium. After spectral filtering, HHG can be considered in the time domain as a source of a train of attosecond pulses which are spaced by half an optical period of the laser field. This characteristic has attracted a lots of interest since it opens the way to attosecond physics. Generating a single attosecond pulse is one of the main challenge. According to simulations, one of the solutions to achieve this goal is to confine the harmonic generation inside a temporal window smaller than one optical cycle of the fundamental laser. In this manuscript, we present a method which allows us to confine the harmonic emission inside a given temporal window and can allow to generate isolated attosecond pulses. This approach relies on the extreme sensitivity of high order harmonic generation on the ellipticity of the fundamental laser field. We developed and analysed a method to modulate temporally the ellipticity of the laser field. To observe the confinement on HHG, we studied, in the first step, the spectral modifications induced by the polarization modulation. In a second step, we performed direct temporal measurements of high order harmonics pulses generated by laser pulses with a time varying polarization. A clear confinement of high harmonic emission is observed. This work also shows that using polarization modulated 10 fs pulses results in the production of an isolated attosecond pulse. To approach this goal, we also developed a new extra-cavity pulse-compression technique suitable for generating high-energy sub-10 femtosecond pulses. (author)
Abstract (French)
Les harmoniques d'ordres eleves, produites lors de l'interaction entre un laser impulsionnel intense et un milieu gazeux, sont emises dans le domaine temporel sous forme d'un train d'impulsions attosecondes espacees d'une demi periode optique du champ laser. La production d'une seule impulsion attoseconde permettrait d'acceder a des resolutions temporelles jusqu'ici inaccessibles pour des etudes resolues en temps. D'apres les simulations, une des solutions pour atteindre cet objectif est de confiner la generation d'harmoniques sur moins d'un cycle optique du laser fondamental. Dans ce manuscrit, nous presentons une methode qui permettrait de restreindre l'emission harmonique a une seule impulsion. Elle repose sur l'extreme sensibilite de la generation d'harmoniques a la polarisation. Nous avons developpe une technique originale permettant de moduler temporellement la polarisation d'une impulsion laser infra-rouge. Dans un premier temps, nous avons etudie les modifications spectrales des harmoniques generees par cette impulsion modulee en polarisation. Dans un second temps, nous avons realise une mesure directe des impulsions harmoniques obtenues en modulant temporellement l'etat de polarisation de l'impulsion laser. Nous avons observe clairement un confinement de la generation d'harmoniques. Ce travail a permis de fixer a environ 10 fs la duree maximale que l'impulsion infrarouge doit avoir pour obtenir une seule impulsion attoseconde. Dans ce cadre, nous avons developpe au laboratoire une technique originale de post-compression d'impulsion laser pour obtenir des impulsions haute energie sub-10 fsFiles
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Additional details
Additional titles
- Original title (French)
- Confinement temporel de la generation d'harmoniques d'ordres eleves
Publishing Information
- Imprint Pagination
- 235 p.
- Report number
- FRCEA-TH--13910
INIS
- Country of Publication
- France
- Country of Input or Organization
- France
- INIS RN
- 53069775
- Subject category
- S74: ATOMIC AND MOLECULAR PHYSICS;
- Resource subtype / Literary indicator
- Thesis
- Descriptors DEI
- EXTREME ULTRAVIOLET RADIATION; FOCUSING; HARMONIC GENERATION; LASERS; NONLINEAR PROBLEMS; SENSITIVITY; TIME RESOLUTION
- Descriptors DEC
- ELECTROMAGNETIC RADIATION; FREQUENCY MIXING; RADIATIONS; RESOLUTION; TIMING PROPERTIES; ULTRAVIOLET RADIATION
Optional Information
- Notes
- 164 refs.; Available from the INIS Liaison Officer for France, see the INIS website for current contact and E-mail addresses