Two-level systems and harmonic excitations in a mean-field anharmonic quantum glass
Creators
- 1. Université Paris-Saclay, CNRS, CEA, Institut de physique théorique, 91191 Gif-sur-Yvette, France
Description
Structural glasses display at low temperature a set of anomalies in thermodynamic observables. A prominent example is the linear-in-temperature scaling of the specific heat, at odds with the Debye cubic scaling found in crystals, due to acoustic phonons. Such an excess of specific heat in amorphous solids is thought of arising from phenomenological soft excitations dubbed tunneling two-level systems (TTLS). Their nature as well as their statistical properties remain elusive from a first-principle viewpoint. In this work, we investigate the canonically quantized version of the KHGPS model, a mean-field glass model of coupled anharmonic oscillators, across its phase diagram, with an emphasis on the specific heat. The thermodynamics is solved in a semiclassical expansion. We show that in the replica-symmetric region of the model, up to the marginal glass transition line where replica symmetry gets continuously broken, a disordered version of the Debye approximation holds: the specific heat is dominated by harmonic vibrational excitations inducing a power-law scaling at the transition, ruled by random matrix theory. This mechanism generalizes a previous semiclassical argument in the literature. We then study the marginal glass phase where the semiclassical expansion becomes nonperturbative due to the emergence of instantons that overcome disordered Debye behavior. Inside the glass phase, a variational solution to the instanton approach provides the prevailing excitations as TTLS, which generate a linear specific heat. This phase thus hosts a mix of TTLS and harmonic excitations generated by interactions. We finally suggest to go beyond the variational approximation through an analogy with the spin-boson model.
Additional details
Identifiers
- DOI
- 10.1103/PhysRevB.110.064203;
- arXiv
- arXiv:2403.12740;
Publishing Information
- Journal Title
- Physical Review B
- Journal Volume
- 110
- Journal Issue
- 6
- Journal Page Range
- 36 pgs.
- ISSN
- 1550-235X
INIS
- Country of Publication
- United States
- Country of Input or Organization
- International Atomic Energy Agency (IAEA)
- Subject category
- S75: CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND SUPERFLUIDITY; S71: CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSICS;
- Descriptors DEI
- AMORPHOUS STATE; CRYSTALS; EXCITATION; EXCITATION SYSTEMS; EXPANSION; GLASS; INSTANTONS; MEAN-FIELD THEORY; PHASE DIAGRAMS; PHONONS; QUANTUM SYSTEMS; RANDOMNESS; SPECIFIC HEAT; SYMMETRY; THERMODYNAMICS; VARIATIONAL METHODS
Optional Information
- Copyright
- ©2024 American Physical Society
- Notes
- Record automatically processed