Published October 10, 2008 | Version v1
Journal article

Tuning the Fragility of a Glass-Forming Liquid by Curving Space

  • 1. Laboratoire de Physique Theorique de la Matiere Condensee, Universite Pierre et Marie Curie-Paris 6, UMR CNRS 7600, 4 place Jussieu, 75252 Paris Cedex 05 (France)

Description

We investigate the influence of space curvature, and of the associated frustration, on the dynamics of a model glass former: a monatomic liquid on the hyperbolic plane. We find that the system's fragility, i.e., the sensitivity of the relaxation time to temperature changes, increases as one decreases the frustration. As a result, curving space provides a way to tune fragility and make it as large as wanted. We also show that the nature of the emerging 'dynamic heterogeneities', another distinctive feature of slowly relaxing systems, is directly connected to the presence of frustration-induced topological defects

Additional details

Publishing Information

Journal Title
Physical Review Letters
Journal Volume
101
Journal Issue
15
Journal Page Range
p. 155701-155701.4
ISSN
0031-9007
CODEN
PRLTAO

INIS

Country of Publication
United States
Country of Input or Organization
International Atomic Energy Agency (IAEA)
INIS RN
40054007
Subject category
S71: CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSICS;
Descriptors DEI
DEFECTS; GLASS; LIQUIDS; RELAXATION TIME; TOPOLOGY
Descriptors DEC
FLUIDS; MATHEMATICS

Optional Information

Notes
(c) 2008 The American Physical Society