Published May 17, 2024 | Version v1
Journal article

Orbital magnetization of a metal is not a bulk property in the mesoscopic regime

  • 1. Materials Science and Engineering, University of California Riverside, Riverside, California 92521, USA
  • 2. Mechanical Engineering, University of California Riverside, Riverside, California 92521, USA

Description

We find that, in the mesoscopic regime, modification of the material's surface can induce an extensive change of the material's magnetic moment. In other words, perturbation of order-N2 atoms on the surface of a three-dimensional solid can change the magnetic moment proportionally to N3. When the solid's surface is perturbed, it triggers two changes in the magnetization. One arises from variations of the electron wave function and energy, while the other arises from a modification in the kinetic angular momentum operator. In the macroscopic regime of our model, these two bulk effects cancel each other, resulting in no impact of the surface perturbation on the magnetization, consistent with prior work. In the mesoscopic regime, we find a departure from this behavior, as the cancellation of two terms is not complete.

Additional details

Identifiers

DOI
10.1103/PhysRevB.109.174431;
arXiv
arXiv:2309.03957;
Crossref Funder ID
10.13039/100000001;

Publishing Information

Journal Title
Physical Review B
Journal Volume
109
Journal Issue
17
Journal Page Range
10 pgs.
ISSN
1550-235X

INIS

Optional Information

Copyright
©2024 American Physical Society
Contract/Grant/Project number
DMR-1848074
Notes
Record automatically processed
Funding organization
National Science Foundation