Published October 20, 2016 | Version v1
Journal article

Nanocluster metal films as thermoelectric material for radioisotope mini battery unit

  • 1. National Research Nuclear University MEPhI (Moscow Engineering Physics Institute), 31 Kashirskoe sh., Moscow 115409 (Russian Federation)
  • 2. Nuclear Safety Institute of Russian Academy of Science, Bolshaya Tulskaya 52, Moscow 115191 (Russian Federation)
  • 3. Skobeltsyn Institute of Nuclear Physics, Lomonosov Moscow State University, Leninskie gory, Moscow 119991 (Russian Federation)
  • 4. Moscow Institute of Physics and Technology (State University), 9 Institutskiy per., Dolgoprudny, Moscow Region 141700 (Russian Federation)

Description

The paper is devoted to studying the thermoelectric and structural properties of films based on metal nanoclusters (Au, Pd, Pt). The experimental results of the study of single nanoclusters' tunneling conductance obtained with scanning tunneling spectroscopy are presented. The obtained data allowed us to evaluate the thermoelectric power of thin film consisting of densely packed individual nanoclusters. It is shown that such thin films can operate as highly efficient thermoelectric materials. A scheme of miniature thermoelectric radioisotope power source based on the thorium-228 isotope is proposed. The efficiency of the radioisotope battery using thermoelectric converters based on nanocluster metal films is shown to reach values up to 1.3%. The estimated characteristics of the device are comparable with the parameters of up-to-date radioisotope batteries based on nickel-63.

Availability note (English)

Available from http://dx.doi.org/10.1016/j.chemphys.2016.07.010

Additional details

Identifiers

DOI
10.1016/j.chemphys.2016.07.010;
PII
S0301-0104(16)30148-3;

Publishing Information

Journal Title
Chemical Physics
Journal Volume
478
Journal Page Range
p. 2-7
ISSN
0301-0104
CODEN
CMPHC2

Optional Information

Copyright
Copyright (c) 2016 Elsevier Science B.V., Amsterdam, The Netherlands, All rights reserved.