Nanocluster metal films as thermoelectric material for radioisotope mini battery unit
Creators
- 1. National Research Nuclear University MEPhI (Moscow Engineering Physics Institute), 31 Kashirskoe sh., Moscow 115409 (Russian Federation)
- 2. Nuclear Safety Institute of Russian Academy of Science, Bolshaya Tulskaya 52, Moscow 115191 (Russian Federation)
- 3. Skobeltsyn Institute of Nuclear Physics, Lomonosov Moscow State University, Leninskie gory, Moscow 119991 (Russian Federation)
- 4. Moscow Institute of Physics and Technology (State University), 9 Institutskiy per., Dolgoprudny, Moscow Region 141700 (Russian Federation)
Description
The paper is devoted to studying the thermoelectric and structural properties of films based on metal nanoclusters (Au, Pd, Pt). The experimental results of the study of single nanoclusters' tunneling conductance obtained with scanning tunneling spectroscopy are presented. The obtained data allowed us to evaluate the thermoelectric power of thin film consisting of densely packed individual nanoclusters. It is shown that such thin films can operate as highly efficient thermoelectric materials. A scheme of miniature thermoelectric radioisotope power source based on the thorium-228 isotope is proposed. The efficiency of the radioisotope battery using thermoelectric converters based on nanocluster metal films is shown to reach values up to 1.3%. The estimated characteristics of the device are comparable with the parameters of up-to-date radioisotope batteries based on nickel-63.
Availability note (English)
Available from http://dx.doi.org/10.1016/j.chemphys.2016.07.010Additional details
Identifiers
- DOI
- 10.1016/j.chemphys.2016.07.010;
- PII
- S0301-0104(16)30148-3;
Publishing Information
- Journal Title
- Chemical Physics
- Journal Volume
- 478
- Journal Page Range
- p. 2-7
- ISSN
- 0301-0104
- CODEN
- CMPHC2
INIS
- Country of Publication
- Netherlands
- Country of Input or Organization
- International Atomic Energy Agency (IAEA)
- INIS RN
- 48093074
- Subject category
- S77: NANOSCIENCE AND NANOTECHNOLOGY;
- Descriptors DEI
- NANOSTRUCTURES; NICKEL 63; RADIOISOTOPE BATTERIES; THERMOELECTRIC CONVERSION; THERMOELECTRIC GENERATORS; THERMOELECTRIC MATERIALS; THIN FILMS; THORIUM 228
- Descriptors DEC
- ACTINIDE NUCLEI; ALPHA DECAY RADIOISOTOPES; BETA DECAY RADIOISOTOPES; BETA-MINUS DECAY RADIOISOTOPES; CONVERSION; DIRECT ENERGY CONVERSION; DIRECT ENERGY CONVERTERS; ENERGY CONVERSION; EVEN-EVEN NUCLEI; EVEN-ODD NUCLEI; FILMS; HEAVY NUCLEI; INTERMEDIATE MASS NUCLEI; ISOTOPES; MATERIALS; NICKEL ISOTOPES; NUCLEI; RADIOISOTOPES; THORIUM ISOTOPES; YEARS LIVING RADIOISOTOPES
Optional Information
- Copyright
- Copyright (c) 2016 Elsevier Science B.V., Amsterdam, The Netherlands, All rights reserved.