Published February 20, 2009 | Version v1
Journal article

First-order dynamical phase transition in models of glasses: an approach based on ensembles of histories

  • 1. School of Physics and Astronomy, University of Nottingham, Nottingham, NG7 2RD (United Kingdom)
  • 2. Department of Chemistry, University of California, Berkeley, CA 94720-1460 (United States)
  • 3. Laboratoire Matiere et Systemes Complexes (CNRS UMR 7057), Universite Paris Diderot, 10 rue Alice Domon et Leonie Duquet, 75205 Paris Cedex 13 (France)
  • 4. Laboratoire des Colloides, Verres et Nanomateriaux (CNRS UMR 5587), Universite de Montpellier II, place Eugene Bataillon, 34095 Montpellier Cedex 5 (France)

Description

We investigate the dynamics of kinetically constrained models of glass formers by analysing the statistics of trajectories of the dynamics, or histories, using large deviation function methods. We show that, in general, these models exhibit a first-order dynamical transition between active and inactive dynamical phases. We argue that the dynamical heterogeneities displayed by these systems are a manifestation of dynamical first-order phase coexistence. In particular, we calculate dynamical large deviation functions, both analytically and numerically, for the Fredrickson-Andersen model, the East model, and constrained lattice gas models. We also show how large deviation functions can be obtained from a Landau-like theory for dynamical fluctuations. We discuss possibilities for similar dynamical phase-coexistence behaviour in other systems with heterogeneous dynamics

Availability note (English)

Available from http://dx.doi.org/10.1088/1751-8113/42/7/075007

Additional details

Identifiers

DOI
10.1088/1751-8113/42/7/075007;
PII
S1751-8113(09)97276-6;

Publishing Information

Journal Title
Journal of Physics. A, Mathematical and Theoretical (Online)
Journal Volume
42
Journal Issue
7
Journal Page Range
[34 p.]
ISSN
1751-8121

INIS

Country of Publication
United Kingdom
Country of Input or Organization
International Atomic Energy Agency (IAEA)
INIS RN
40074900
Subject category
S71: CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSICS;
Descriptors DEI
FLUCTUATIONS; FUNCTIONS; GLASS; PHASE TRANSFORMATIONS; STATISTICS; TRAJECTORIES
Descriptors DEC
MATHEMATICS; VARIATIONS