Published June 2007 | Version v1
Journal article

Anomalous magnetic phase in an undistorted pyrochlore oxide Cd2Os2O7 induced by geometrical frustration

  • 1. High Energy Accelerator Research Organization, Institute of Materials Structure Science, Tsukuba, Ibaraki (Japan)
  • 2. Japan Atomic Energy Agency, Advanced Science Research Center, Tokai, Ibaraki (Japan)
  • 3. Tokyo Univ., Inst. for Solid State Physics, Kashiwa, Chiba (JP)

Description

We report on the muon spin rotation/relaxation study of a pyrochlore oxide, Cd2Os2O7, which exhibits a metal-insulator (MI) transition at TMI ≅ 225 K without structural phase transition. It reveals strong spin fluctuation (≥108 s-1) below the MI transition, suggesting a predominant role of geometrical spin frustration amongst Os5+ ions. Meanwhile, upon further cooling, an incommensurate spin density wave discontinuously develops below TSDW ≅ 150 K. These observations strongly suggest the occurrence of an anomalous magnetic transition and associated change in the local spin dynamics in undistorted pyrochlore antiferromagnet. (author)

Additional details

Publishing Information

Journal Title
Journal of the Physical Society of Japan
Journal Volume
76
Journal Issue
6
Journal Page Range
p. 063703.1-063703.4
ISSN
0031-9015

Optional Information

Notes
21 refs., 4 figs.